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具有对称性破缺的全介质q-BIC超表面的光学手性

Optical chirality of all dielectric q-BIC metasurface with symmetry breaking.

作者信息

Sun Yujia, He Chongjun, Deng Zilan, Li Xin, Li Xiaozhi, Zhang Zhongyuan, Sui Xiubao, Li Ning, He Weiji, Chen Fangzhou

机构信息

College of Astronautics, Nanjing University of Aeronautics and Astronautics, Nanjing 211106, China.

Guangdong Provincial Key Laboratory of Optical Fiber Sensing and Communications, Institute of Photonics Technology, College of Physics & Optoelectronic Engineering, Jinan University, Guangzhou 510632, China.

出版信息

Nanophotonics. 2025 Mar 17;14(5):559-569. doi: 10.1515/nanoph-2024-0666. eCollection 2025 Mar.

Abstract

As a two-dimensional material at the nanoscale, optical metasurfaces have excellent and flexible optical field control methods. In particular, the application of the concept of bound states in the continuum (BIC) enables optical metasurfaces to achieve resonance effects with high quality factors (Q factor). In comparison to plasmonic metasurfaces, all dielectric metasurfaces can effectively reduce the Ohmic losses in the structure. In this study, we propose a q-BIC metasurface with a high quality factor (maximum Q factor of 247), which is all dielectric and symmetry-breaking, and investigate the enhancement effect of this structure on optical chirality in the near-infrared band. In the simulation and experiment, the transmission spectra of the structure in the near-infrared band exhibited differences at different light source incidence angles when illuminated with circularly polarised light of varying rotation directions (external chirality). The maximum far-field circular dichroism (CD) achieved was 0.17 in the simulation and 0.038 in the experiment. Subsequently, the near-field chirality enhancement of the structure was investigated, which has the potential to increase the optical chirality of the incident light by up to 22 times. Furthermore, the introduction of a chiral medium to a non-chiral metasurface results in a chiral transfer effect, enabling the achievement of circular dichroism beyond the intrinsic capabilities of the individual substances involved (maximum CD = 0.0055). The high-Q factor of the all-dielectric metasurface paves the way for a plenty of potential applications in optical chiral fields, including chiral sensing, ultra-sensitive analysis of biomaterials and soft matter.

摘要

作为一种纳米级的二维材料,光学超表面具有出色且灵活的光场控制方法。特别是,连续域束缚态(BIC)概念的应用使光学超表面能够实现具有高品质因数(Q因子)的共振效应。与等离子体超表面相比,全介质超表面可以有效降低结构中的欧姆损耗。在本研究中,我们提出了一种具有高品质因数(最大Q因子为247)的q-BIC超表面,它是全介质且破缺对称性的,并研究了这种结构在近红外波段对光学手性的增强作用。在模拟和实验中,当用不同旋转方向(外在手性)的圆偏振光照射时,该结构在近红外波段的透射光谱在不同光源入射角下表现出差异。模拟中实现的最大远场圆二色性(CD)为0.17,实验中为0.038。随后,研究了该结构的近场手性增强,其有可能将入射光的光学手性提高多达22倍。此外,将手性介质引入非手性超表面会产生手性转移效应,从而能够实现超越所涉及单个物质固有能力的圆二色性(最大CD = 0.0055)。全介质超表面的高Q因子为光学手性领域的大量潜在应用铺平了道路,包括手性传感、生物材料和软物质的超灵敏分析。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8b03/11953724/c0f960afbc70/j_nanoph-2024-0666_fig_001.jpg

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