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强耦合实现的手性激光发射

Chiral lasing enabled by strong coupling.

作者信息

Deng Huachun, Jiang Xiong, Zhang Yao, Zeng Yixuan, Barkaoui Hamdi, Xiao Shumin, Yu Shaohua, Kivshar Yuri, Song Qinghai

机构信息

Ministry of Industry and Information Technology Key Lab of Micro-Nano Optoelectronic Information System, Guangdong Provincial Key Laboratory of Semiconductor Optoelectronic Materials and Intelligent Photonic Systems, Harbin Institute of Technology, Shenzhen 518055, P. R. China.

Pengcheng Laboratory, Shenzhen 518055, P. R. China.

出版信息

Sci Adv. 2025 Apr 11;11(15):eads9562. doi: 10.1126/sciadv.ads9562. Epub 2025 Apr 9.

Abstract

Chiral quasi-bound states in the continuum are spin-dependent high- resonances in meta-photonic structures that are realized by perturbing symmetry-protected optical states by engineering in-plane and out-of-plane asymmetries, and they support chiral lasing in the vertical direction. Here, we explore the coupling between two resonances in a chiral metasurface and introduce a mechanism for high-purity chiral laser emission. We reveal that two resonances with nearly orthogonal polarizations become strongly coupled in an engineered chiral metasurface. The inherent phase difference of the resonances, associated with the coherent destruction on the decay channel, can endow high- factor and maximize chirality to one of the hybrid modes. We verify this approach experimentally by measuring transmission spectra, angle-resolved photoluminescence, and laser emission. We believe that this mechanism allows breaking restrictions on conventional chiral quasi-BIC lasing, enabling the realization of chiral emission at any designed direction.

摘要

连续统中的手性准束缚态是超光子结构中与自旋相关的高共振态,通过设计面内和面外不对称性来扰动对称性保护的光学态来实现,并且它们在垂直方向上支持手性激光发射。在此,我们探索手性超表面中两个共振之间的耦合,并引入一种实现高纯度手性激光发射的机制。我们揭示了在设计的手性超表面中,两个具有近乎正交偏振的共振会强烈耦合。共振的固有相位差与衰变通道上的相干破坏相关,可赋予其中一个混合模式高因子并使手性最大化。我们通过测量透射光谱、角分辨光致发光和激光发射,对该方法进行了实验验证。我们相信,这种机制能够突破传统手性准束缚态激光发射的限制,实现任意设计方向上的手性发射。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/dc0f/11980839/5e200912e744/sciadv.ads9562-f1.jpg

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