Worku Michael, Ben-Akacha Azza, Blessed Shonde Tunde, Liu He, Ma Biwu
Materials Science and Engineering Program Florida State University Tallahassee FL 32306 USA.
Department of Chemistry and Biochemistry Florida State University Tallahassee FL 32306 USA.
Small Sci. 2021 May 7;1(8):2000072. doi: 10.1002/smsc.202000072. eCollection 2021 Aug.
Metal halide perovskites (MHPs) have emerged as new-generation highly efficient narrow-band luminescent materials with applications in various optoelectronic devices, including photovoltaics (PVs), light-emitting diodes (LEDs), lasers, and scintillators. Since the demonstration of efficient room-temperature electroluminescence from MHPs in 2014, remarkable progress has been achieved in the development and study of light-emitting MHP materials and devices. While the device efficiencies of MHP LEDs (PeLEDs) have significantly improved over a short period of time, their overall performance has not reached the levels of mature technologies yet, such as organic LEDs (OLEDs) and quantum dot LEDs (QDLEDs), to enable practical applications. Many issues and challenges, including low operational stability, lack of efficient blue PeLEDs, and toxicity of MHPs, remain to be addressed. Herein, some of the most exciting progress achieved in the development of efficient and stable PeLEDs during the last few years are introduced, the main issues and challenges in the field are discussed, and the prospects on addressing these issues and challenges are provided. With continuous effort, the potential of PeLEDs to become a commercially available LED technology for display and lighting applications in the future looks optimistic.
金属卤化物钙钛矿(MHPs)已成为新一代高效窄带发光材料,应用于各种光电器件,包括光伏(PVs)、发光二极管(LEDs)、激光器和闪烁体。自2014年展示出金属卤化物钙钛矿在室温下的高效电致发光以来,发光金属卤化物钙钛矿材料及器件的开发与研究取得了显著进展。尽管金属卤化物钙钛矿发光二极管(PeLEDs)的器件效率在短时间内有了显著提高,但其整体性能尚未达到有机发光二极管(OLEDs)和量子点发光二极管(QDLEDs)等成熟技术的水平,无法实现实际应用。许多问题和挑战依然存在,包括操作稳定性低、缺乏高效蓝色PeLEDs以及金属卤化物钙钛矿的毒性等。本文介绍了过去几年在高效稳定PeLEDs开发方面取得的一些最令人振奋的进展,讨论了该领域的主要问题和挑战,并展望了解决这些问题和挑战的前景。通过持续努力,PeLEDs未来成为用于显示和照明应用的商用LED技术的潜力看起来很乐观。