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纳赛尔湖水的放射风险及其对健康和环境的影响。

Radiological risks in Nasser lake water and their health and environmental implications.

作者信息

Ali Khaled, Abu-Taleb Ahmed, Abbady Abd El-Baset, Harb Shaban

机构信息

Physics Department, Faculty of Science, South Valley University, Qena, Egypt.

出版信息

Sci Rep. 2025 Apr 25;15(1):14545. doi: 10.1038/s41598-025-95257-7.

DOI:10.1038/s41598-025-95257-7
PMID:40281049
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC12031930/
Abstract

This study aimed to evaluate the activity concentrations of naturally occurring radionuclides (NORs) in Nasser Lake water, assess the associated radiological risks, and investigate the potential health and environmental impacts. The presence of these NORs is attributed to both natural geological formations, such as uranium-rich granitic and metamorphic rocks, and anthropogenic activities, including agricultural runoff. Water samples were analyzed for radium-226 (Ra-226), thorium-232 (Th-232), and potassium-40 (K-40). The Ra-226 concentration ranged from 0.08 ± 0.003 to 1.28 ± 0.06 becquerel per liter (Bq/l), mostly between 0.2 and 1.0 Bq/l, reflecting geological and anthropogenic influences. The symbol (±) represents the measurement uncertainty associated with gamma spectrometric analysis. According to international radiation safety guidelines, Ra-226 levels below 1 Bq/l are considered safe for consumption. The Th-232 concentration varied from 0.04 ± 0.001 to 0.96 ± 0.06 Bq/l, showing significant spatial variation. Similarly, K-40 concentrations ranged from 1.35 ± 0.11 to 16.57 ± 1.43 Bq/l, with some notably high values. The annual effective dose (E) ranged from 15.8 to 266.15 micro sievert per year (µSv/y) for adults, reaching 362.92 µSv/y for children and 221.54 µSv/y for infants. The doses for children and infants exceeded the recommended thresholds. Cancer risk (CR) assessments showed that men's mortality risks ranged from 2.56 × 10 to 4.10 × 10, while women's ranged from 2.68 × 10 to 4.29 × 10. Morbidity risks varied between 3.72 × 10 and 5.95 × 10 for men and 3.89 × 10 to 6.22 × 10 for women. These risks correlate with specific lake locations, highlighting hot spots with elevated radioactive content. Water acidity levels (pH) ranged from 6.23 to 7.9, indicating predominantly neutral to slightly alkaline conditions. These variations correlated with electrical conductivity (EC), reflecting complex interaction between pH, EC, and NORs. The study assesses gamma radiation hazards from external exposure and internal risks from alpha-emitting radionuclides, such as Ra-226 and Th-232, through water ingestion. While most samples comply with standard radiation limits, elevated radionuclide levels in certain areas pose potential health risks, particularly for vulnerable populations like children. Continuous monitoring of radiological parameters in Naser Lake is essential to trace long-term trends and ensure safety compliance. Additionally, advanced water treatment methods could help mitigate radionuclide concentrations in affected areas.

摘要

本研究旨在评估纳赛尔湖水中天然存在的放射性核素(NORs)的活度浓度,评估相关的辐射风险,并调查其对健康和环境的潜在影响。这些NORs的存在归因于天然地质构造,如富含铀的花岗岩和变质岩,以及人为活动,包括农业径流。对水样进行了镭 - 226(Ra - 226)、钍 - 232(Th - 232)和钾 - 40(K - 40)的分析。Ra - 226浓度范围为每升0.08±0.003至1.28±0.06贝克勒尔(Bq/l),大多在0.2至1.0 Bq/l之间,反映了地质和人为影响。符号(±)表示与伽马能谱分析相关的测量不确定度。根据国际辐射安全准则,低于1 Bq/l的Ra - 226水平被认为对消费是安全的。Th - 232浓度从0.04±0.001至0.96±0.06 Bq/l不等,显示出显著的空间变化。同样,K - 40浓度范围为1.35±0.11至16.57±1.43 Bq/l,有一些明显的高值。成人的年有效剂量(E)范围为每年15.8至266.15微希沃特(µSv/y),儿童达到362.92 µSv/y,婴儿为221.54 µSv/y。儿童和婴儿的剂量超过了推荐阈值。癌症风险(CR)评估表明,男性的死亡风险范围为2.56×10至4.10×10,而女性为2.68×10至4.29×10。男性的发病风险在3.72×10至5.95× 10之间,女性在3.89×10至6.22×10之间。这些风险与特定的湖泊位置相关,突出了放射性含量升高的热点区域。水的酸度水平(pH)范围为6.23至7.9,表明主要为中性至微碱性条件。这些变化与电导率(EC)相关,反映了pH、EC和NORs之间的复杂相互作用。该研究评估了外部暴露的伽马辐射危害以及通过饮水摄入镭 - 226和钍 - 232等发射α粒子的放射性核素带来的内部风险。虽然大多数样本符合标准辐射限值,但某些地区放射性核素水平升高带来了潜在的健康风险,特别是对儿童等弱势群体。持续监测纳赛尔湖的放射学参数对于追踪长期趋势和确保符合安全标准至关重要。此外,先进的水处理方法有助于降低受影响地区的放射性核素浓度。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/541b/12031930/0e0815fd3fd6/41598_2025_95257_Fig5_HTML.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/541b/12031930/0e0815fd3fd6/41598_2025_95257_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/541b/12031930/b6dcb4b61ce4/41598_2025_95257_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/541b/12031930/4893e191a882/41598_2025_95257_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/541b/12031930/14970a2ddfd5/41598_2025_95257_Fig3_HTML.jpg
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Methods for radioactivity measurements in drinking water using gamma spectrometry.用伽马谱法测量饮用水放射性的方法。
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