Jia Qisong, Ye Wenhao, Zhang Chang, Jia Zhuoyi, Liu Ji, Wang Tongchao, Zhao Liupeng, Liu Yongshun, Wang Chen, Sun Peng, Fan Zhiyong, Lu Geyu
State Key Laboratory of Integrated Optoelectronics (JLU Region), College of Electronic Science and Engineering, Jilin University, Changchun 130012, China.
Department of Electronic and Computer Engineering, The Hong Kong University of Science and Technology, Clear Water Bay, Kowloon, Hong Kong SAR 999077, China.
Nano Lett. 2025 Jun 18;25(24):9726-9733. doi: 10.1021/acs.nanolett.5c01881. Epub 2025 Jun 4.
Wearable sensors are advancing personalized healthcare and environmental safety, yet integrating multimodal sensing remains challenging due to material incompatibility, cross-sensitivity, and environmental interference. To address this gap, we present a monolithic wristband-integrated multimodal sensing platform for simultaneous environmental and physiological monitoring. The system integrates sensors for NO, UV irradiance, epidermal temperature, and human pulse signals. A TiO/WS heterojunction-based resistive transduction matrix, as the core sensing material, achieves room-temperature NO detection (theoretical limit of detection of 14.4 ppb) with 12-month stability, UV intensity measurement (0.024-1.68 mW/cm), epidermal temperature monitoring (25-50 °C, sensitivity of 0.22%/°C), and arterial pulse waveform analysis (P-T-D peak resolution). A hybrid neuroevolutionary algorithm (GA-BP) decouples photo-gas interference, reducing quantification errors to <3.5%. Flexible electronics and selective encapsulation (PDMS, PET shielding) ensure mechanical durability and accurate signal acquisition. The platform demonstrates multifunctional capabilities that enable point-of-care health and environmental monitoring, bridging personalized diagnostics with exposure assessment.
可穿戴传感器正在推动个性化医疗保健和环境安全的发展,然而,由于材料不相容、交叉敏感性和环境干扰,集成多模态传感仍然具有挑战性。为了填补这一空白,我们提出了一种用于同时进行环境和生理监测的单片腕带集成多模态传感平台。该系统集成了用于检测一氧化氮(NO)、紫外线辐照度、表皮温度和人体脉搏信号的传感器。以TiO/WS异质结为基础的电阻式传感矩阵作为核心传感材料,可实现室温下的NO检测(理论检测极限为14.4 ppb),具有12个月的稳定性,可测量紫外线强度(0.024 - 1.68 mW/cm)、监测表皮温度(25 - 50°C,灵敏度为0.22%/°C)以及分析动脉脉搏波形(P - T - D峰值分辨率)。一种混合神经进化算法(GA - BP)可消除光气干扰,将定量误差降低至<3.5%。柔性电子器件和选择性封装(PDMS、PET屏蔽)确保了机械耐久性和准确的信号采集。该平台展示了多功能能力,能够实现即时医疗健康和环境监测,将个性化诊断与暴露评估联系起来。