Chen Jinli, Cui Chaohan, Lawrie Ben, Xue Yongzhou, Guha Saikat, Eichenfield Matt, Zhao Huan, Yan Xiaodong
Department of Materials Science and Engineering, University of Arizona, Tucson, AZ 85721, USA.
Department of Electrical and Computer Engineering, University of Maryland, College Park, MD 20742, USA.
Nanophotonics. 2025 Jan 8;14(11):1687-1713. doi: 10.1515/nanoph-2024-0569. eCollection 2025 Jun.
Solid-state single-photon emitters (SPEs) are attracting significant attention as fundamental components in quantum computing, communication, and sensing. Low-dimensional materials-based SPEs (LD-SPEs) have drawn particular interest due to their high photon extraction efficiency, ease of integration with photonic circuits, and strong coupling with external fields. The accessible surfaces of LD materials allow for deterministic control over quantum light emission, while enhanced quantum confinement and light-matter interactions improve photon emissive properties. This perspective examines recent progress in LD-SPEs across four key materials: zero-dimensional (0D) semiconductor quantum dots, one-dimensional (1D) nanotubes, two-dimensional (2D) materials, including hexagonal boron nitride (hBN) and transition metal dichalcogenides (TMDCs). We explore their structural and photophysical properties, along with techniques such as spectral tuning and cavity coupling, which enhance SPE performance. Finally, we address future challenges and suggest strategies for optimizing LD-SPEs for practical quantum applications.
固态单光子发射器(SPEs)作为量子计算、通信和传感中的基础组件,正吸引着广泛关注。基于低维材料的单光子发射器(LD-SPEs)因其高光子提取效率、易于与光子电路集成以及与外部场的强耦合而备受关注。低维材料的可及表面允许对量子发光进行确定性控制,而增强的量子限制和光与物质的相互作用改善了光子发射特性。本文综述了基于四种关键材料的LD-SPEs的最新进展:零维(0D)半导体量子点、一维(1D)纳米管、二维(2D)材料,包括六方氮化硼(hBN)和过渡金属二硫属化物(TMDCs)。我们探讨了它们的结构和光物理性质,以及诸如光谱调谐和腔耦合等增强SPE性能的技术。最后,我们讨论了未来的挑战,并提出了优化LD-SPEs以用于实际量子应用的策略。