Di Giulio Valerio, Haindl Rudolf, Ropers Claus
Department of Ultrafast Dynamics, Max Planck Institute for Multidisciplinary Sciences, D-37077 Göttingen, Germany.
4th Physical Institute - Solids and Nanostructures, Georg-August-Universität Göttingen, D-37077 Göttingen, Germany.
Nanophotonics. 2025 May 22;14(11):1865-1878. doi: 10.1515/nanoph-2025-0040. eCollection 2025 Jun.
Nonclassical states of light are fundamental in various applications, spanning quantum computation to enhanced sensing. Fast free electrons, which emit light into photonic structures through the mechanism of spontaneous emission, represent a promising platform for generating diverse types of states. Indeed, the intrinsic connection between the input electron wave function and the output light field suggests that electron-shaping schemes, based on light-induced scattering, facilitate their synthesis. In this article, we present a theoretical framework capable of predicting the final optical density matrix emitted by a generic -electron state that can also account for post-sample energy filtering. By using such a framework, we study the modulation-dependent fluctuations of the -electron emission and identify regions of superradiant scaling characterized by Poissonian and super-Poissonian statistics. In this context, we predict that high- modulated electron pulses can yield a tenfold shot-noise suppression in the estimation of the electron-light coupling when the output radiation intensity is analyzed. In the single-electron case, we show how coherent states with nearly 90 % purity can be formed by pre-filtering a portion of the spectrum after modulation, and how non-Gaussian states are generated after a precise energy measurement. Furthermore, we present a strategy combining a single-stage electron modulation and post-filtering to harness tailored light states, such as squeezed vacuum, cat, and triangular cat states, with fidelities close to 100 %.
非经典光态在从量子计算到增强传感等各种应用中至关重要。快速自由电子通过自发发射机制将光发射到光子结构中,是产生多种类型光态的一个有前景的平台。实际上,输入电子波函数与输出光场之间的内在联系表明,基于光致散射的电子整形方案有助于光态的合成。在本文中,我们提出了一个理论框架,该框架能够预测由一般电子态发射的最终光密度矩阵,并且还能考虑样品后的能量过滤。通过使用这样的框架,我们研究了电子发射的调制相关涨落,并确定了以泊松统计和超泊松统计为特征的超辐射标度区域。在此背景下,我们预测当分析输出辐射强度时,高调制电子脉冲在估计电子 - 光耦合时可实现十倍的散粒噪声抑制。在单电子情况下,我们展示了如何通过在调制后对一部分光谱进行预滤波来形成纯度接近90%的相干态,以及在精确能量测量后如何产生非高斯态。此外,我们提出了一种结合单级电子调制和后滤波的策略,以利用保真度接近100%的定制光态,如压缩真空态、猫态和三角猫态。