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由二维金红石和MXene ScCF组成的合理设计的多功能异质结构。

Rationally Designed Versatile Heterostructures Consisted of Two-Dimensional Goldene and MXene ScCF.

作者信息

Nguyen Chuong V, Truong Pham Thiet, Phuc Huynh V, Nguyen Cuong Q, Hiep Nguyen T, Hieu Nguyen N

机构信息

Department of Materials Science and Engineering, Le Quy Don Technical University, Hanoi 100000, Vietnam.

Faculty of Physics, Hue University of Education, Hue University, Hue 530000, Vietnam.

出版信息

Nano Lett. 2025 Jul 2;25(26):10673-10679. doi: 10.1021/acs.nanolett.5c02560. Epub 2025 Jun 18.

DOI:10.1021/acs.nanolett.5c02560
PMID:40531925
Abstract

The rational design of two-dimensional (2D) metal-semiconductor (M-S) heterostructures through contact engineering is crucial for the development of next-generation nanoelectronic devices. In this Letter, van der Waals design strategies were employed to explore the contact characteristics between goldene and MXene ScCF. Our findings reveal that n-type Schottky contacts are formed across all goldene/ScCF heterostructures. Notably, this heterostructure exhibits reversible switching between n- and p-type Schottky contacts and can be tuned from Schottky to ohmic contacts via electric gating and vertical strain. Furthermore, goldene/ScCF exhibits a low tunneling specific resistivity of 2.80 × 10 Ω cm, indicating its excellent charge injection efficiency. These findings offer valuable theoretical guidance for the design and optimization of goldene-based devices, such as field-effect transistors (FETs) and photodetectors.

摘要

通过接触工程对二维(2D)金属 - 半导体(M - S)异质结构进行合理设计对于下一代纳米电子器件的发展至关重要。在本信函中,采用范德华设计策略来探究金烯与MXene ScCF之间的接触特性。我们的研究结果表明,在所有金烯/ScCF异质结构中均形成了n型肖特基接触。值得注意的是,这种异质结构在n型和p型肖特基接触之间表现出可逆切换,并且可以通过电门控和垂直应变从肖特基接触调谐为欧姆接触。此外,金烯/ScCF表现出2.80×10Ω·cm的低隧穿比电阻率,表明其具有优异的电荷注入效率。这些发现为基于金烯的器件(如场效应晶体管(FET)和光电探测器)的设计和优化提供了有价值的理论指导。

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