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二维磁体FeGeTe中由几何诱导应变稳定的局域自旋纹理

Localized Spin Textures Stabilized by Geometry-Induced Strain in 2D Magnet FeGeTe.

作者信息

Sun Yuhan, Birch Max T, Finizio Simone, Powalla Lukas, Satheesh Sayooj, Priessnitz Tim, Göring Eberhard, Knöckl Ernst, Kastl Christoph, Holleitner Alexander, Kern Klaus, Weigand Markus, Wintz Sebastian, Burghard Marko

机构信息

Max Planck Institute for Solid State Research, Heisenbergstrasse 1, 70569, Stuttgart, Germany.

RIKEN Center for Emergent Matter Science, Wako, 351-0198, Japan.

出版信息

Adv Mater. 2025 Sep;37(37):e2506279. doi: 10.1002/adma.202506279. Epub 2025 Jun 18.

DOI:10.1002/adma.202506279
PMID:40534280
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC12447047/
Abstract

Strain engineering promises to enable manipulation and control of the properties of exfoliated flakes of 2D van der Waals (vdW) ferromagnets for spintronic applications. However, while previous studies of strain effects have focused on global properties, the impact on local magnetic spin textures remains unexplored. Here, manipulation of magnetism in the 2D ferromagnet FeGeTe (FGT) is demonstrated using geometry-induced strain. Employing scanning transmission X-ray microscopy (STXM), the effects of spatially varying strain profiles on the magnetic order of FGT sheets stamped onto micropillar arrays are directly visualized. It is found that the in-plane strain components, with magnitudes <0.5%, locally elevate the Curie temperature of FGT by 10 K, stabilizing magnetic domains near the pillar corners. These domains include skyrmions and higher-order topological spin textures such as skyrmioniums and skyrmion bags. The possibility to locally seed and control topological spin textures via strain opens new avenues for future spin-based information technologies.

摘要

应变工程有望实现对二维范德华(vdW)铁磁体剥离薄片特性的操纵和控制,以用于自旋电子学应用。然而,尽管先前关于应变效应的研究集中在全局特性上,但对局部磁自旋纹理的影响仍未得到探索。在此,利用几何诱导应变展示了对二维铁磁体FeGeTe(FGT)磁性的操纵。采用扫描透射X射线显微镜(STXM),直接可视化了空间变化的应变分布对压印在微柱阵列上的FGT薄片磁序的影响。研究发现,面内应变分量大小<0.5%,局部将FGT的居里温度提高了10 K,稳定了柱角附近的磁畴。这些磁畴包括斯格明子以及高阶拓扑自旋纹理,如斯格明子团和斯格明子袋。通过应变局部播种和控制拓扑自旋纹理的可能性为未来基于自旋的信息技术开辟了新途径。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4c67/12447047/c4637ede46a7/ADMA-37-2506279-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4c67/12447047/c8389fa46edb/ADMA-37-2506279-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4c67/12447047/1fea0657d55e/ADMA-37-2506279-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4c67/12447047/c5e4ec82f739/ADMA-37-2506279-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4c67/12447047/01c53f93f66a/ADMA-37-2506279-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4c67/12447047/c4637ede46a7/ADMA-37-2506279-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4c67/12447047/c8389fa46edb/ADMA-37-2506279-g006.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4c67/12447047/1fea0657d55e/ADMA-37-2506279-g001.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4c67/12447047/c5e4ec82f739/ADMA-37-2506279-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4c67/12447047/01c53f93f66a/ADMA-37-2506279-g005.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4c67/12447047/c4637ede46a7/ADMA-37-2506279-g003.jpg

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本文引用的文献

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Superconducting diode effect under time-reversal symmetry.时间反演对称性下的超导二极管效应
Sci Adv. 2024 Aug 2;10(31):eado1502. doi: 10.1126/sciadv.ado1502. Epub 2024 Jul 31.
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Topological Spin Textures: Basic Physics and Devices.拓扑自旋纹理:基础物理与器件
Adv Mater. 2025 Jan;37(2):e2312935. doi: 10.1002/adma.202312935. Epub 2024 Jul 1.
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Voltage control of magnetism in FeGeTe/InSe van der Waals ferromagnetic/ferroelectric heterostructures.FeGeTe/InSe范德华铁磁/铁电异质结构中磁性的电压控制
Nat Commun. 2023 Sep 12;14(1):5605. doi: 10.1038/s41467-023-41382-8.
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Strain Engineering of Intrinsic Ferromagnetism in 2D van der Waals Materials.二维范德华材料本征铁磁性的应变工程
Nanomaterials (Basel). 2023 Aug 19;13(16):2378. doi: 10.3390/nano13162378.
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Emerging Spintronic Materials and Functionalities.新兴的自旋电子材料与功能
Adv Mater. 2024 May;36(22):e2301854. doi: 10.1002/adma.202301854. Epub 2023 Nov 3.
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