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使用量子气体激光雷达测量澳大利亚昆士兰州一个废弃煤炭勘探孔的甲烷逸散排放。

Measurement of fugitive methane emissions from an abandoned coal exploration hole in Queensland, Australia using a Quantum Gas LiDAR.

作者信息

Hoerning Sebastian, Hayes Philip

机构信息

Gas & Energy Transition Research Centre, The University of Queensland, Brisbane, 4072, Queensland, Australia.

Gas & Energy Transition Research Centre, The University of Queensland, Brisbane, 4072, Queensland, Australia.

出版信息

Sci Total Environ. 2025 Aug 25;992:179925. doi: 10.1016/j.scitotenv.2025.179925. Epub 2025 Jun 29.

DOI:10.1016/j.scitotenv.2025.179925
PMID:40587932
Abstract

Rapid reduction in global methane emissions has been identified as the fastest approach to reduce future global warming and emission reduction requires accurate identification of sources, and reliable emission quantification. This study addresses an unaccounted source of methane by providing the first longer-term quantification of substantial fugitive methane emissions from an abandoned coal exploration borehole in Queensland, Australia, revealing a mean emission rate of 235 t/a. Depending on the Global Warming Potential applied, this mean rate is equivalent to 6580 or 19,768 t COe. The surveyed borehole, classified as a "super-emitter" (>25 kg/h), exhibited substantial temporal variability in methane flux with the 5th and 95th percentile of 22.8 t/a and 438 t/a, respectively. The survey used a trailer mounted Quantum Gas LiDAR system to enable continuous monitoring over seven days and six nights in variable weather conditions. Exploratory data analysis identified a negative correlation with atmospheric pressure as a likely meteorological driver of emission rate variability, although other factors such as subsurface (groundwater) pressure changes may also influence emission rates. The study highlights that legacy coal exploration infrastructure, if improperly sealed, can act as anthropogenic pathways for uncontrolled methane release. These findings indicate the need for surveys of a larger sample of coal exploration holes across Queensland's coal basins to understand the frequency and rates of emissions, to investigate emissions from other holes, such as water bores, and further investigation of emission dynamics considering geological characteristics and nearby activities. This research indicates the possible significance of legacy coal exploration bores as an under-reported and unaccounted source of methane emissions, with potential implications for coal basins globally.

摘要

全球甲烷排放量的快速减少已被确定为减缓未来全球变暖的最快途径,而减排需要准确识别排放源并进行可靠的排放量量化。本研究通过首次对澳大利亚昆士兰州一个废弃煤炭勘探钻孔大量逃逸甲烷排放进行长期量化,解决了一个未被核算的甲烷排放源问题,结果显示平均排放率为235吨/年。根据所应用的全球变暖潜势,这一平均排放率相当于6580或19768吨二氧化碳当量。被归类为“超级排放源”(>25千克/小时)的被调查钻孔,其甲烷通量呈现出显著的时间变化,第5百分位数和第95百分位数分别为22.8吨/年和438吨/年。该调查使用了一个安装在拖车上的量子气体激光雷达系统,以便在多变的天气条件下进行连续七天六夜的监测。探索性数据分析确定,与大气压力呈负相关可能是排放率变化的一个气象驱动因素,不过诸如地下(地下水)压力变化等其他因素也可能影响排放率。该研究强调,如果密封不当,遗留的煤炭勘探基础设施可能成为甲烷无控制释放的人为通道。这些发现表明,需要对昆士兰州煤炭盆地更大样本的煤炭勘探钻孔进行调查,以了解排放频率和速率,调查其他钻孔(如水井)的排放情况,并结合地质特征和附近活动进一步研究排放动态。这项研究表明,遗留的煤炭勘探钻孔作为一个未被充分报告和核算的甲烷排放源可能具有重要意义,对全球煤炭盆地可能产生影响。

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