Xie Tian, Wolf Tobias M, Xu Siyuan, Cui Zhiyuan, Xiong Richen, Ou Yunbo, Hays Patrick, Holleis Ludwig F, Guo Yi, Sheekey Owen I, Patterson Caitlin, Arp Trevor, Watanabe Kenji, Taniguchi Takashi, Tongay Seth Ariel, Young Andrea F, MacDonald Allan H, Jin Chenhao
Department of Physics, University of California at Santa Barbara, Santa Barbara, CA, USA.
Department of Physics, University of Texas at Austin, Austin, TX, USA.
Nat Commun. 2025 Jul 1;16(1):5555. doi: 10.1038/s41467-025-60675-8.
Spin- and valley flavor polarization plays a central role in the many-body physics of flat band graphene, with Fermi surface reconstruction - often accompanied by quantized anomalous Hall and superconducting state - observed in a variety of experimental systems. Here we describe an optical technique that sensitively and selectively detects flavor textures via the exciton response of a proximal transition metal dichalcogenide layer. Through a systematic study of rhombohedral and rotationally faulted graphene bilayers and trilayers, we show that when the semiconducting dichalcogenide is in direct contact with the graphene, the exciton response is most sensitive to the large momentum rearrangement of the Fermi surface, providing information that is distinct from and complementary to electrical compressibility measurements. The wide-field imaging capability of optical probes allows us to obtain spatial maps of flavor order with high throughput, and with broad temperature and device compatibility. Our work helps pave the way for optical probing and imaging of flavor orders in flat band graphene systems.
自旋和谷味极化在平带石墨烯的多体物理中起着核心作用,在各种实验系统中都观察到了费米面重构,通常伴随着量子化反常霍尔效应和超导态。在此我们描述一种光学技术,它通过近端过渡金属二硫族化物层的激子响应灵敏且选择性地检测味纹理。通过对菱形和旋转断层石墨烯双层及三层的系统研究,我们表明当半导体二硫族化物与石墨烯直接接触时,激子响应对费米面的大动量重排最为敏感,提供了与电压缩性测量不同且互补的信息。光学探针的宽场成像能力使我们能够以高通量获得味序的空间图,并具有广泛的温度和器件兼容性。我们的工作有助于为平带石墨烯系统中味序的光学探测和成像铺平道路。