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反铁磁材料中的章动共振模式。

Nutational resonance modes in antiferromagnetic materials.

作者信息

Angster David, Dannegger Tobias, Schlegel Julius, Evers Martin, Nowak Ulrich

机构信息

Fachbereich Physik, Universität Konstanz, D-78457, Konstanz, Germany.

出版信息

Sci Rep. 2025 Jul 1;15(1):21543. doi: 10.1038/s41598-025-08746-0.

DOI:10.1038/s41598-025-08746-0
PMID:40596594
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC12214598/
Abstract

The Landau-Lifshitz-Gilbert (LLG) equation is well-established to describe the spin dynamics of magnetic materials. This first-order differential equation is based on the assumption that the spin angular momenta and corresponding magnetic moments are always parallel. While this assumption is largely unproblematic, both theoretical considerations and experimental results have indicated that the two may become separated on ultrafast timescales, giving rise to inertial dynamics along with a modified spin wave dispersion. Here, we apply linear spin wave theory to the inertial LLG equation to compute the eigenmodes of the altermagnetic materials SmErFeO and α-FeO. We find the largest influence of nutation on the magnetic resonances in the case of hematite, which exhibits both a sizeable shift of the resonance frequencies as compared to the inertia-free case and additional nutational resonances that are in a similar order of magnitude to the materials' higher-frequency precessional exchange modes. While the realistic magnitude of the inertial parameter remains an open question, we hope that our quantitative analysis provides the starting point for further experimental investigations.

摘要

朗道-栗弗席兹-吉尔伯特(LLG)方程已被广泛用于描述磁性材料的自旋动力学。这个一阶微分方程基于自旋角动量和相应磁矩始终平行的假设。虽然这个假设在很大程度上没有问题,但理论考量和实验结果都表明,在超快时间尺度上,两者可能会分离,从而产生惯性动力学以及修正的自旋波色散。在此,我们将线性自旋波理论应用于惯性LLG方程,以计算交替磁性材料SmErFeO和α-FeO的本征模。我们发现,在赤铁矿的情况下,章动对磁共振的影响最大,与无惯性情况相比,其共振频率有相当大的偏移,并且还有额外的章动共振,其量级与材料的高频进动交换模式相似。虽然惯性参数的实际大小仍然是一个悬而未决的问题,但我们希望我们的定量分析能为进一步的实验研究提供起点。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c8d/12214598/e61b63074c5c/41598_2025_8746_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c8d/12214598/f3824a4715b1/41598_2025_8746_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c8d/12214598/805f2e711342/41598_2025_8746_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c8d/12214598/ce58bbdbe88d/41598_2025_8746_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c8d/12214598/c81d6de3f3f9/41598_2025_8746_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c8d/12214598/a5ece3d30d58/41598_2025_8746_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c8d/12214598/e61b63074c5c/41598_2025_8746_Fig6_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c8d/12214598/f3824a4715b1/41598_2025_8746_Fig1_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c8d/12214598/805f2e711342/41598_2025_8746_Fig2_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c8d/12214598/ce58bbdbe88d/41598_2025_8746_Fig3_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c8d/12214598/c81d6de3f3f9/41598_2025_8746_Fig4_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c8d/12214598/a5ece3d30d58/41598_2025_8746_Fig5_HTML.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/2c8d/12214598/e61b63074c5c/41598_2025_8746_Fig6_HTML.jpg

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本文引用的文献

1
Discovery of ultrafast spontaneous spin switching in an antiferromagnet by femtosecond noise correlation spectroscopy.通过飞秒噪声关联光谱法在反铁磁体中发现超快自发自旋切换。
Nat Commun. 2023 Nov 29;14(1):7651. doi: 10.1038/s41467-023-43318-8.
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Inertial Spin Dynamics in Epitaxial Cobalt Films.外延钴薄膜中的惯性自旋动力学
Phys Rev Lett. 2022 Dec 2;129(23):237201. doi: 10.1103/PhysRevLett.129.237201.
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Anisotropic long-range spin transport in canted antiferromagnetic orthoferrite YFeO.倾斜反铁磁正铁氧体YFeO₃中的各向异性长程自旋输运
Nat Commun. 2022 Oct 17;13(1):6140. doi: 10.1038/s41467-022-33520-5.
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Long-distance spin-transport across the Morin phase transition up to room temperature in ultra-low damping single crystals of the antiferromagnet α-FeO.在反铁磁体α-FeO的超低阻尼单晶中,跨越莫林相变直至室温的长距离自旋输运。
Nat Commun. 2020 Dec 10;11(1):6332. doi: 10.1038/s41467-020-20155-7.
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Anisotropic and nonlinear magnetodielectric effects in orthoferrite ErFeO single crystals.正铁氧体ErFeO单晶中的各向异性和非线性磁电效应
Sci Rep. 2020 Jul 16;10(1):11825. doi: 10.1038/s41598-020-68800-x.
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