Chen Song, Wu Zumin, Wei Lei, Bai Xiuqin, Yuan Chengqing, Guo Zhiwei, Yang Ying
College of Mechanical Engineering, Hunan Institute of Science and Technology, Yueyang 414006, China.
School of Life Science, Keele University, Stoke-on-Trent ST4 7QB, UK.
Gels. 2025 Jul 7;11(7):526. doi: 10.3390/gels11070526.
Both biosystems and engineering fields demand advanced friction-reducing and lubricating materials. Due to their hydrophilicity and tissue-mimicking properties, hydrogels are ideal candidates for use as lubricants in water-based environments. They are particularly well-suited for applications involving biocompatibility or interactions with intelligent devices such as soft robots. However, external environments, whether within the human body or in engineering applications, often present a wide range of dynamic conditions, including variations in shear stress, temperature, light, pH, and electric fields. Additionally, hydrogels inherently possess low mechanical strength, and their dimensional stability can be compromised by changes during hydration. This review focuses on recent advancements in using environmentally responsive hydrogels as lubricants. It explores strategies involving physical or structural modifications, as well as the incorporation of smart chemical functional groups into hydrogel polymer chains, which enable diverse responsive mechanisms. Drawing on both the existing literature and our own research, we also examine how composite friction materials where hydrogels serve as water-based lubricants offer promising solutions for demanding engineering environments, such as bearing systems in marine vessels.
生物系统和工程领域都需要先进的减摩和润滑材料。由于水凝胶具有亲水性和组织模拟特性,它们是在水基环境中用作润滑剂的理想选择。它们特别适合涉及生物相容性或与软机器人等智能设备相互作用的应用。然而,无论是在人体内部还是在工程应用中,外部环境通常呈现出广泛的动态条件,包括剪切应力、温度、光照、pH值和电场的变化。此外,水凝胶本身机械强度较低,其尺寸稳定性可能会因水化过程中的变化而受到影响。本综述重点关注使用环境响应性水凝胶作为润滑剂的最新进展。它探讨了涉及物理或结构改性的策略,以及将智能化学官能团引入水凝胶聚合物链的策略,这些策略能够实现多种响应机制。结合现有文献和我们自己的研究,我们还研究了以水凝胶作为水基润滑剂的复合摩擦材料如何为苛刻的工程环境(如船舶轴承系统)提供有前景的解决方案。