Lee Jooseop, Chappell Greta L, Baumbach Ryan E, Said Ayman H, Zaliznyak Igor A
Hongik University, Department of Science, Seoul 04066, Republic of Korea.
CALDES, Institute for Basic Science, Pohang 37673, Republic of Korea.
Phys Rev Lett. 2025 Jul 18;135(3):036705. doi: 10.1103/clg4-2zzb.
Using high-energy-resolution inelastic x-ray scattering, we observe anomalous softening and damping of the transverse acoustic phonon in UPt_{2}Si_{2} as the system is cooled toward the charge density wave (CDW) transition temperature T_{CDW}. The phonon exhibits a marked Kohn-type anomaly around the CDW wave vector Q_{CDW} and becomes overdamped within a finite momentum range already well above T_{CDW}. The dispersion anomaly is consistent with potential Fermi surface nesting, which together with the extended phonon collapse indicates strong electron-phonon coupling. The transition temperature estimated from the phonon softening is markedly lower than T_{CDW}, consistent with a primarily electronic instability rather than a phonon-driven transition. Our results establish UPt_{2}Si_{2} as a prime example of a strongly correlated electron CDW system with exceptionally strong electron-phonon coupling driving phonon softening and collapse.
利用高能分辨率非弹性X射线散射,我们观察到,当系统冷却至电荷密度波(CDW)转变温度TCDW时,UPt2Si2中横向声学声子出现反常软化和阻尼现象。在CDW波矢QCDW附近,声子呈现出显著的科恩型反常,并且在远高于TCDW的有限动量范围内就变成了过阻尼状态。色散反常与潜在的费米面嵌套相一致,这与扩展的声子崩塌一起表明了强电子-声子耦合。由声子软化估计出的转变温度明显低于TCDW,这与主要是电子不稳定性而非声子驱动的转变相一致。我们的结果表明,UPt2Si2是强关联电子CDW系统的一个典型例子,具有异常强的电子-声子耦合,驱动声子软化和崩塌。