Wang Hui, Gupta Adit, Lu Qiuchun, Wu Wenting, Wang Xueyang, Huang Xin, Hu Xuanyi, Lee Pooi See
School of Materials Science and Engineering, Nanyang Technological University, Singapore, Singapore.
Nat Commun. 2025 Aug 11;16(1):7405. doi: 10.1038/s41467-025-62796-6.
Dielectric elastomer actuators (DEAs) exhibit large actuation strains, lightweight, and fast response, making them a promising candidate for soft robotics and soft grippers. Ionogels have been used as the electrodes in DEAs to offer thermostability and self-healability, however, typically the elastic modulus of the self-healing ionogel electrodes is of several tens of kPa (or higher), limiting the actuation strain performance and self-healing speed of the DEA. In this work, a poly(ionic liquid) (PIL) electrode with an ultralow elastic modulus of 3.4 kPa and rapid self-healing within 10 s in ambient and underwater conditions is achieved through ionic interaction regulation. The resultant DEAs realized an area strain of 63.2%, and maintained the strains after 10 s of self-healing at room temperature, outperforming other reported DEAs with self-healing electrodes. With the PIL electrode, a soft gripper composed of two bending DEAs is fabricated to gently handle soft and delicate objects in both air and underwater settings, retaining functionality even after damages due to self-healing of the PIL electrodes. The PIL electrode advances the development of electrically driven soft robotics for exploration in harsh environment or underwater settings.
介电弹性体致动器(DEAs)具有大的驱动应变、轻质和快速响应的特点,使其成为软机器人和软夹爪的有前途的候选者。离子凝胶已被用作DEAs中的电极以提供热稳定性和自修复性,然而,通常自修复离子凝胶电极的弹性模量为几十千帕(或更高),这限制了DEA的驱动应变性能和自修复速度。在这项工作中,通过离子相互作用调节实现了一种超低弹性模量为3.4 kPa且在环境和水下条件下10 s内快速自修复的聚离子液体(PIL)电极。所得的DEAs实现了63.2%的面积应变,并在室温下自修复10 s后保持应变,优于其他报道的带有自修复电极的DEAs。使用PIL电极,制造了一个由两个弯曲DEAs组成的软夹爪,用于在空气和水下环境中轻柔地处理柔软易碎的物体,即使在因PIL电极自修复而受损后仍能保持功能。PIL电极推动了用于在恶劣环境或水下环境中探索的电动软机器人的发展。