Stegani Nadia, Pallecchi Ilaria, Manca Nicola, Meinero Martina, Iebole Michela, Cialone Matteo, Braccini Valeria, Karmakar Koushik, Maljuk Andrey, Büchner Bernd, Grinenko Vadim, Putti Marina, Caglieris Federico
Department of Physics, University of Genoa, Genoa, Italy.
Consiglio Nazionale delle Ricerche (CNR)-SPIN, Genoa, Italy.
Sci Technol Adv Mater. 2025 Aug 21;26(1):2546282. doi: 10.1080/14686996.2025.2546282. eCollection 2025.
The spontaneous Hall effect (SHE), a finite voltage occurring transversal to the electrical current in zero-magnetic field, has been observed in both conventional and unconventional superconductors, appearing as a peak near the superconducting transition temperature. The origin of SHE is strongly debated, with proposed explanations ranging from intrinsic and extrinsic mechanisms such as spontaneous symmetry breaking and time-reversal symmetry breaking (BTRS), Abrikosov vortex motion, or extrinsic factors like material inhomogeneities, such as non-uniform critical temperature (T) distributions or structural asymmetries. This work is an experimental study of the SHE in various superconducting materials. We focused on conventional, low-T, sharp transition Nb and unconventional, intermediate-Tc, smeared transition Fe(Se,Te). Our findings show distinct SHE peaks around the superconducting transition, with variations in height, sign and shape, indicating a possible common mechanism independent of the specific material. We propose that spatial inhomogeneities in the critical temperature, caused by local chemical composition variations, disorder, or other forms of electronic spatial inhomogeneities could explain the appearance of the SHE. This hypothesis is supported by comprehensive finite elements simulations of randomly distributed Tc's by varying T-distribution, spatial scale of disorder and amplitude of the superconducting transition. The comparison between experimental results and simulations suggests a unified origin for the SHE in different superconductors, whereas different phenomenology can be explained in terms of amplitude of the transition temperature with respect to Tc-distribution.
自发霍尔效应(SHE)是指在零磁场中,与电流方向垂直出现的有限电压,在传统和非传统超导体中均有观测到,表现为超导转变温度附近的一个峰值。SHE的起源存在激烈争论,提出的解释包括内在和外在机制,如自发对称性破缺和时间反演对称性破缺(BTRS)、阿布里科索夫涡旋运动,或外在因素,如材料不均匀性,如临界温度(T)分布不均匀或结构不对称。这项工作是对各种超导材料中SHE的实验研究。我们聚焦于传统的、低T、尖锐转变的铌以及非传统的、中Tc、弥散转变的Fe(Se,Te)。我们的研究结果表明,在超导转变附近有明显的SHE峰值,其高度、符号和形状存在变化,这表明可能存在一种与特定材料无关的共同机制。我们提出,由局部化学成分变化、无序或其他形式的电子空间不均匀性引起的临界温度空间不均匀性可以解释SHE的出现。通过改变T分布、无序的空间尺度和超导转变的幅度对随机分布的Tc进行全面的有限元模拟,支持了这一假设。实验结果与模拟结果的比较表明,不同超导体中SHE有统一的起源,而不同的现象学可以用相对于Tc分布的转变温度幅度来解释。