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From efficiency to sustainability: organic additives for interfacial regulation in lithium metal batteries.

作者信息

Gu Wei, He Di, Qin Yuting, Fu Chongchong, Lu Jiahui, Wang Tianyi, Wang Guoxiu, Sun Bing

机构信息

School of Chemistry and Chemical Engineering, Yangzhou University Yangzhou 225002 P. R. China

Centre for Clean Energy Technology, School of Mathematical and Physical Sciences, Faculty of Science, University of Technology Sydney Sydney NSW 2007 Australia

出版信息

Chem Sci. 2025 Sep 15. doi: 10.1039/d5sc03975d.

DOI:10.1039/d5sc03975d
PMID:41019644
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC12466591/
Abstract

The utilization of lithium (Li) metal anodes is gaining renewed attention due to the increasing demand for electric vehicles (EVs) and the continuous rise in traditional energy consumption. These Li metal anodes exhibit a high theoretical discharge capacity (3860 mAh g) and an ultra-low redox potential (-3.04 V the SHE), making them the coveted "Holy Grail" for next-generation lithium-ion batteries (LIBs). However, challenges in terms of uncontrolled formation of Li dendrites, instability in the solid electrolyte interphases (SEI) layer, and numerous parasitic reactions have hindered the commercialization of Li metal anodes. In recent years, extensive research has been conducted on the appropriate utilization of organic additives as a long-term, stable, cost-effective, and practical approach to enhancing their stability. The present review investigates the effects of various types and molecular weights of organic additives on the preservation of Li metal anodes and their influence on SEI membrane modification. Finally, we offer valuable insights into the prospective development trajectory of organic additives that are compatible with Li metal anodes.

摘要
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/4ca7/12466591/4e54a0d4b7d9/d5sc03975d-p4.jpg
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