Brudvig G W, Stevens T H, Chan S I
Biochemistry. 1980 Nov 11;19(23):5275-85. doi: 10.1021/bi00564a020.
The reactions of nitric oxide (NO) with both oxidized and reduced cytochrome c oxidase are reported. NMR and mass spectroscopy were utilized to determine the products of the reactions; EPR and optical spectroscopy were employed to determine the states of the enzyme produced in each of these reactions. It was found that the enzyme catalyzes the consecutive oxidation and reduction of NO. A different cycle was observed when NO was added to the reduced enzyme, to the oxidized enzyme, or to the oxidized enzyme in the presence of azide. It was possible to observe the state of the enzyme at several points in each of these three cycles by varying the concentration of NO. The reactions of NO all involved a one- or two-electron redox step and could be accounted for by the involvement of only cytochrome a3 and Cua3. On the basis of these results, a mechanism for the reduction of dioxygen by the enzyme is proposed in which cytochrome a3 functions to anchor dioxygen and intermediates while remaining in the ferrous state, whereas Cua3 functions to accept electroins from cytochrome a/Cua and transfer them to dioxygen.
报道了一氧化氮(NO)与氧化型和还原型细胞色素c氧化酶的反应。利用核磁共振(NMR)和质谱来确定反应产物;采用电子顺磁共振(EPR)和光谱学来确定这些反应中产生的酶的状态。发现该酶催化NO的连续氧化和还原。当向还原型酶、氧化型酶或在叠氮化物存在下的氧化型酶中添加NO时,观察到不同的循环。通过改变NO的浓度,可以在这三个循环的每个循环中的几个点观察酶的状态。NO的反应均涉及单电子或双电子氧化还原步骤,并且仅由细胞色素a3和Cua3的参与即可解释。基于这些结果,提出了该酶还原双氧的机制,其中细胞色素a3在保持亚铁状态的同时起到锚定双氧和中间体的作用,而Cua3起到从细胞色素a/Cua接受电子并将其转移至双氧的作用。