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Structure of bacteriochlorophyll aggregates in chlorosomes of green bacteria: a spectral hole burning study.

作者信息

Novoderezhkin V I, Fetisova Z G

机构信息

A.N. Belozersky Institute of Physico-Chemical Biology, Moscow State University, Russia.

出版信息

Biochem Mol Biol Int. 1996 Oct;40(2):243-52. doi: 10.1080/15216549600201732.

DOI:10.1080/15216549600201732
PMID:8896746
Abstract

Exciton level structure, homogenous absorption and hole-burning spectra were calculated for different models of bacteriochlorophyll aggregation in chlorosomal antennae of green bacteria. It was demonstrated that none of the earlier proposed models of noninteracting linear bacteriochlorophyll aggregates and linear bacteriochlorophyll chains assembling in tubular aggregates with high density of packing, exhibits the in vivo exciton level structure revealed by hole-burning experiments on intact cells of green bacteria. The models of linear exciton-coupled bacteriochlorophyll chains with a low packing density, approximating that in vivo, were proposed as alternative, to obtain the main spectral features found in natural antennae.

摘要

相似文献

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引用本文的文献

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Exciton dynamics in the chlorosomal antenna of the green bacterium Chloroflexus aurantiacus: experimental and theoretical studies of femtosecond pump-probe spectra.橙色绿弯菌叶绿体天线中的激子动力学:飞秒泵浦-探测光谱的实验与理论研究
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