Moody A J, Mitchell R, Jeal A E, Rich P R
Glynn Research Foundation, Glynn, Bodmin, Cornwall PL30 4AU, U.K.
Biochem J. 1997 Jun 15;324 ( Pt 3)(Pt 3):743-52. doi: 10.1042/bj3240743.
The binding of four anionic ligands, cyanide, fluoride, azide and formate, to cytochrome bo purified from Escherichia coli cells grown with a copper supplement (+Cu cyt.bo) is described. Membrane-bound cytochrome bo that lacks the copper component, CuB, of its active site can be prepared from cells grown under conditions where the availability of copper is limited by the presence of a CuI chelator, 2,2'-bicinchinonic acid. The ligand-binding properties of this copper-less enzyme (-Cu cyt.bo) are compared with those of +Cu cyt. bo. As judged from near-UV/visible spectroscopic changes, cyanide forms a low-spin complex with +Cu cyt.bo, whereas azide, fluoride and formate form high-spin complexes. The pH-dependences of binding suggest that for all four of these anionic ligands, both the rates of binding and the binding affinities are primarily dependent on the concentration of their protonated forms. -Cu cyt.bo, which shows less than 15% of the duroquinol oxidase activity of +Cu cyt.bo, binds cyanide, azide and fluoride, but with greatly decreased affinity (<1/30, 1/2000 and 1/2500 respectively at pH5.5 compared with +Cu cyt.bo). The complex of azide with -Cu cyt.bo still seems to be high-spin and azide binding to -Cu cyt.bo is still pH-dependent, although less so than azide binding to +Cu cyt.bo.
本文描述了四种阴离子配体,即氰化物、氟化物、叠氮化物和甲酸盐,与从添加了铜的大肠杆菌细胞中纯化得到的细胞色素bo(+Cu cyt.bo)的结合情况。膜结合的细胞色素bo缺乏其活性位点的铜组分CuB,可以从在铜的可用性受CuI螯合剂2,2'-联喹啉酸限制的条件下生长的细胞中制备。将这种无铜酶(-Cu cyt.bo)的配体结合特性与+Cu cyt.bo的进行了比较。从近紫外/可见光谱变化判断,氰化物与+Cu cyt.bo形成低自旋复合物,而叠氮化物、氟化物和甲酸盐形成高自旋复合物。结合的pH依赖性表明,对于所有这四种阴离子配体,结合速率和结合亲和力主要取决于它们质子化形式的浓度。-Cu cyt.bo的杜罗醌醇氧化酶活性不到+Cu cyt.bo的15%,它能结合氰化物、叠氮化物和氟化物,但亲和力大大降低(在pH5.5时,与+Cu cyt.bo相比分别小于1/30、1/2000和1/2500)。叠氮化物与-Cu cyt.bo的复合物似乎仍然是高自旋的,并且叠氮化物与-Cu cyt.bo的结合仍然依赖于pH,尽管程度低于叠氮化物与+Cu cyt.bo的结合。