Hemming C, Kapral R
Chemical Physics Theory Group, Department of Chemistry, University of Toronto, Toronto, ON M5S 3H6, Canada.
Faraday Discuss. 2001(120):371-82; discussion 407-19. doi: 10.1039/b103237m.
Phase fronts in the forced complex Ginzburg-Landau equation, a model of a resonantly forced oscillatory reaction-diffusion system, are studied in the 3:1 resonance regime. The focus is on the turbulent (Benjamin-Feir-unstable) regime of the corresponding unforced system; in the forced system, phase fronts between spatially uniform phase-locked states exhibit complex dynamics. In one dimension, for strong forcing, phase fronts move with constant velocity. As the forcing intensity is lowered there is a bifurcation to oscillatory motion, followed by a bifurcation to a regime in which fronts multiply via the nucleation of domains of the third homogeneous phase in the front. In two dimensional systems, rough fronts with turbulent, complex internal structure may arise. For a critical value of the forcing intensity there is a nonequilibrium phase transition in which the turbulent interface grows to occupy the entire system. The phenomena we explore can be probed by experiments on periodically forced light sensitive reaction-diffusion systems.
在3:1共振状态下,研究了受迫复金兹堡-朗道方程中的相位前沿,该方程是一个共振受迫振荡反应扩散系统的模型。重点在于相应无受迫系统的湍流(本杰明-费尔不稳定)状态;在受迫系统中,空间均匀锁相状态之间的相位前沿呈现出复杂的动力学。在一维情况下,对于强驱动,相位前沿以恒定速度移动。随着驱动强度降低,会出现向振荡运动的分岔,随后又会出现一个分岔,进入一种前沿通过前沿中第三均匀相区域的成核而增殖的状态。在二维系统中,可能会出现具有湍流、复杂内部结构的粗糙前沿。对于驱动强度的一个临界值,会发生非平衡相变,其中湍流界面增长并占据整个系统。我们所探索的现象可以通过对周期性受迫的光敏反应扩散系统进行实验来探究。