Woycechowsky Kenneth J, Hook Brad A, Raines Ronald T
Department of Biochemistry and Department of Chemistry, University of Wisconsin-Madison, Madison, Wisconsin 53706, USA.
Biotechnol Prog. 2003 Jul-Aug;19(4):1307-14. doi: 10.1021/bp0257123.
The isomerization of non-native disulfide bonds often limits the rate of protein folding. Small-molecule dithiols can catalyze this process. Here, a symmetric trithiol, tris(2-mercaptoacetamidoethyl)amine, is designed on the basis of criteria known to be important for efficient catalysis of oxidative protein folding. The trithiol is synthesized and attached to two distinct solid supports via one of its three sulfhydryl groups. The resulting immobilized dithiol has an apparent disulfide E degrees ' = -208 mV, which is close to that of protein disulfide isomerase (E degrees ' = -180 mV). Incubation of the dithiol immobilized on a TentaGel resin with a protein containing non-native disulfide bonds produced only a 2-fold increase in native protein. This dithiol appeared to be inaccessible to protein. In contrast, incubation of the dithiol immobilized on styrene-glycidyl methacrylate microspheres with the non-native protein produced a 17-fold increase in native protein. This increase was 1.5-fold greater than that of a monothiol immobilized on the microspheres. Thus, the choice of both the solid support and thiol can affect catalysis of protein folding. The use of dithiol-decorated microspheres is an effective new strategy for preparative protein folding in vitro.
非天然二硫键的异构化常常限制蛋白质折叠的速率。小分子二硫醇能够催化这一过程。在此,基于已知对氧化蛋白质折叠高效催化很重要的标准设计了一种对称三硫醇,即三(2-巯基乙酰氨基乙基)胺。合成该三硫醇并通过其三个巯基之一连接到两种不同的固体支持物上。所得的固定化二硫醇的表观二硫键E°' = -208 mV,这与蛋白质二硫键异构酶的E°'(-180 mV)接近。将固定在TentaGel树脂上的二硫醇与含有非天然二硫键的蛋白质一起温育,天然蛋白质仅增加了2倍。这种二硫醇似乎无法与蛋白质接触。相比之下,将固定在苯乙烯-甲基丙烯酸缩水甘油酯微球上的二硫醇与非天然蛋白质一起温育,则天然蛋白质增加了17倍。这一增加比固定在微球上的单硫醇的增加大1.5倍。因此,固体支持物和硫醇的选择均可影响蛋白质折叠的催化作用。使用二硫醇修饰的微球是体外制备性蛋白质折叠的一种有效的新策略。