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空气采样器收集的木屑气溶胶粒径分布比较。

Comparison of wood-dust aerosol size-distributions collected by air samplers.

作者信息

Harper Martin, Akbar Muhammad Zabed, Andrew Michael E

机构信息

National Institute for Occupational Safety and Health, MS-3030 1095 Willowdale Rd, Morgantown, WV 26505, USA.

出版信息

J Environ Monit. 2004 Jan;6(1):18-22. doi: 10.1039/b312883k. Epub 2003 Dec 5.

Abstract

A method has been described previously for determining particle size distributions in the inhalable size range collected by personal samplers for wood dust. In this method, the particles collected by a sampler are removed, suspended, and re-deposited on a mixed cellulose-ester filter, and examined by optical microscopy to determine particle aerodynamic diameters. This method is particularly appropriate to wood-dust particles which are generally large and close to rectangular prisms in shape. The method was used to investigate the differences in total mass found previously in studies of side-by-side sample collection with different sampler types. Over 200 wood-dust samples were collected in three different wood-products industries, using the traditional 37 mm closed-face polystyrene/acrylonitrile cassette (CFC), the Institute of Occupational Medicine (IOM) inhalable sampler, and the Button sampler developed by the University of Cincinnati. Total mass concentration results from the samplers were found to be in approximately the same ratio as those from traditional long-term gravimetric samples, but about an order of magnitude higher. Investigation of the size distributions revealed several differences between the samplers. The wood dust particulate mass appears to be concentrated in the range 10-70 aerodynamic equivalent diameter (AED), but with a substantial mass contribution from particles larger than 100 microm AED in a significant number of samples. These ultra-large particles were found in 65% of the IOM samples, 42% of the CFC samples and 32% of the Button samples. Where present, particles of this size range dominated the total mass collected, contributing an average 53% (range 10-95%). However, significant differences were still found after removal of the ultra-large particles. In general, the IOM and CFC samplers appeared to operate in accordance with previous laboratory studies, such that they both collected similar quantities of particles at the smaller diameters, up to about 30-40 [micro sign]m AED, after which the CFC collection efficiency was reduced dramatically compared to the IOM. The Button sampler collected significantly less than the IOM at particle sizes between 10.1 and 50 microm AED. The collection efficiency of the Button sampler was significantly different from that of the CFC for particle sizes between 10.1 and 40 microm AED, and the total mass concentration given by the Button sampler was significantly less than that given by the CFC, even in the absence of ultra-large particles. The results are consistent with some relevant laboratory studies.

摘要

先前已描述了一种用于确定通过个人采样器收集的可吸入粒径范围内木尘颗粒大小分布的方法。在该方法中,将采样器收集的颗粒取出、悬浮,然后重新沉积在混合纤维素酯滤膜上,并通过光学显微镜检查以确定颗粒的空气动力学直径。该方法特别适用于通常较大且形状接近长方体的木尘颗粒。该方法用于研究先前在不同采样器类型的并排采样研究中发现的总质量差异。在三个不同的木制品行业中,使用传统的37毫米封闭面聚苯乙烯/丙烯腈盒式采样器(CFC)、职业医学研究所(IOM)可吸入采样器和辛辛那提大学开发的纽扣采样器收集了200多个木尘样本。发现采样器的总质量浓度结果与传统长期重量法样本的结果大致成相同比例,但大约高一个数量级。对粒径分布的研究揭示了采样器之间的几个差异。木尘颗粒质量似乎集中在空气动力学等效直径(AED)为10 - 70的范围内,但在大量样本中,粒径大于100微米AED的颗粒对总质量有相当大的贡献。在65%的IOM样本、42%的CFC样本和32%的纽扣样本中发现了这些超大颗粒。在存在此类颗粒的情况下,该粒径范围内的颗粒占收集到的总质量的主导地位,平均贡献53%(范围为10% - 95%)。然而,在去除超大颗粒后仍发现了显著差异。一般来说,IOM和CFC采样器的运行似乎与先前的实验室研究一致,即它们在较小直径(高达约30 - 40微米AED)下收集的颗粒数量相似,此后与IOM相比,CFC的收集效率大幅降低。在粒径为10.1至50微米AED之间时,纽扣采样器收集的颗粒明显少于IOM。在粒径为10.1至40微米AED之间时,纽扣采样器的收集效率与CFC的收集效率显著不同,并且即使在没有超大颗粒的情况下,纽扣采样器给出的总质量浓度也明显低于CFC给出的总质量浓度。这些结果与一些相关的实验室研究一致。

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