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测量单根碳纳米管的热导率。

Measuring the thermal conductivity of a single carbon nanotube.

作者信息

Fujii Motoo, Zhang Xing, Xie Huaqing, Ago Hiroki, Takahashi Koji, Ikuta Tatsuya, Abe Hidekazu, Shimizu Tetsuo

机构信息

Institute for Materials Chemistry and Engineering, Kyushu University, Kasuga 816-8580, Japan.

出版信息

Phys Rev Lett. 2005 Aug 5;95(6):065502. doi: 10.1103/PhysRevLett.95.065502. Epub 2005 Aug 2.

Abstract

Although the thermal properties of millimeter-sized carbon nanotube mats and packed carbon nanofibers have been readily measured, measurements for a single nanotube are extremely difficult. Here, we report a novel method that can reliably measure the thermal conductivity of a single carbon nanotube using a suspended sample-attached T-type nanosensor. Our experimental results show that the thermal conductivity of a carbon nanotube at room temperature increases as its diameter decreases, and exceeds 2000 W/mK for a diameter of 9.8 nm. The temperature dependence of the thermal conductivity for a carbon nanotube with a diameter of 16.1 nm appears to have an asymptote near 320 K. The present method is, in principle, applicable to any kind of a single nanofiber, nanowire, and even single-walled carbon nanotube.

摘要

尽管毫米尺寸的碳纳米管垫和填充碳纳米纤维的热性能已易于测量,但对单个纳米管的测量却极其困难。在此,我们报告一种新颖的方法,该方法可使用附着有悬浮样品的T型纳米传感器可靠地测量单个碳纳米管的热导率。我们的实验结果表明,室温下碳纳米管的热导率随其直径减小而增加,对于直径为9.8 nm的碳纳米管,其热导率超过2000 W/mK。直径为16.1 nm的碳纳米管的热导率与温度的关系在320 K附近似乎有一条渐近线。本方法原则上适用于任何种类的单个纳米纤维、纳米线,甚至单壁碳纳米管。

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