Noti Christian, de Paz Jose L, Polito Laura, Seeberger Peter H
Laboratory for Organic Chemistry, Swiss Federal Institute of Technology ETH Zürich, Wolfgang-Pauli-Strasse 10, HCI F315, 8093 Zürich, Switzerland.
Chemistry. 2006 Nov 24;12(34):8664-86. doi: 10.1002/chem.200601103.
Heparin is a highly sulfated, linear polymer that participates in a plethora of biological processes by interaction with many proteins. The chemical complexity and heterogeneity of this polysaccharide can explain the fact that, despite its widespread medical use as an anticoagulant drug, the structure-function relationship of defined heparin sequences is still poorly understood. Here, we present the chemical synthesis of a library containing heparin oligosaccharides ranging from di- to hexamers of different sequences and sulfation patterns. An amine-terminated linker was placed at the reducing end of the synthetic structures to allow for immobilization onto N-hydroxysuccinimide activated glass slides and creation of heparin microarrays. Key features of this modular synthesis, such as the influence of the amine linker on the glycosidation efficiency, the use of 2-azidoglucose as glycosylating agents for oligosaccharide assembly, and the compatibility of the protecting group strategy with the sulfation-deprotection steps, are discussed. Heparin microarrays containing this oligosaccharide library were constructed using a robotic printer and employed to characterize the carbohydrate binding affinities of three heparin-binding growth factors. FGF-1, FGF-2 and FGF-4 that are implicated in angiogenesis, cell growth and differentiation were studied. These heparin chips aided in the discovery of novel, sulfated sequences that bind FGF, and in the determination of the structural requirements needed for recognition by using picomoles of protein on a single slide. The results presented here highlight the potential of combining oligosaccharide synthesis and carbohydrate microarray technology to establish a structure-activity relationship in biological processes.
肝素是一种高度硫酸化的线性聚合物,通过与许多蛋白质相互作用参与众多生物过程。这种多糖的化学复杂性和异质性可以解释这样一个事实,即尽管肝素作为抗凝血药物在医学上广泛应用,但其特定序列的结构 - 功能关系仍知之甚少。在此,我们展示了一个包含不同序列和硫酸化模式的二聚体至六聚体肝素寡糖文库的化学合成。在合成结构的还原端放置了一个胺基末端连接子,以便固定在N - 羟基琥珀酰亚胺活化的载玻片上并创建肝素微阵列。讨论了这种模块化合成的关键特征,例如胺连接子对糖苷化效率的影响、使用2 - 叠氮葡萄糖作为寡糖组装的糖基化试剂以及保护基策略与硫酸化 - 去保护步骤的兼容性。使用机器人打印机构建了包含该寡糖文库的肝素微阵列,并用于表征三种肝素结合生长因子的碳水化合物结合亲和力。研究了与血管生成、细胞生长和分化有关的FGF - 1、FGF - 2和FGF - 4。这些肝素芯片有助于发现与FGF结合的新型硫酸化序列,并通过在单个载玻片上使用皮摩尔级别的蛋白质来确定识别所需的结构要求。此处呈现的结果突出了结合寡糖合成和碳水化合物微阵列技术以在生物过程中建立结构 - 活性关系的潜力。