Djurisić Aleksandra B, Leung Yu Hang
Department of Physics, The University of Hong Kong, Pokfulam Road, Hong Kong.
Small. 2006 Aug;2(8-9):944-61. doi: 10.1002/smll.200600134.
We present a review of current research on the optical properties of ZnO nanostructures. We provide a brief introduction to different fabrication methods for various ZnO nanostructures and some general guidelines on how fabrication parameters (temperature, vapor-phase versus solution-phase deposition, etc.) affect their properties. A detailed discussion of photoluminescence, both in the UV region and in the visible spectral range, is provided. In addition, different gain (excitonic versus electron hole plasma) and feedback (random lasing versus individual nanostructures functioning as Fabry-Perot resonators) mechanisms for achieving stimulated emission are described. The factors affecting the achievement of stimulated emission are discussed, and the results of time-resolved studies of stimulated emission are summarized. Then, results of nonlinear optical studies, such as second-harmonic generation, are presented. Optical properties of doped ZnO nanostructures are also discussed, along with a concluding outlook for research into the optical properties of ZnO.
我们对当前关于ZnO纳米结构光学性质的研究进行了综述。我们简要介绍了各种ZnO纳米结构的不同制备方法,以及制备参数(温度、气相沉积与溶液相沉积等)如何影响其性质的一些一般指导原则。提供了对紫外区域和可见光谱范围内光致发光的详细讨论。此外,还描述了实现受激发射的不同增益(激子与电子空穴等离子体)和反馈(随机激光与作为法布里-珀罗谐振器的单个纳米结构)机制。讨论了影响实现受激发射的因素,并总结了受激发射的时间分辨研究结果。然后,展示了非线性光学研究的结果,如二次谐波产生。还讨论了掺杂ZnO纳米结构的光学性质,并对ZnO光学性质的研究进行了总结展望。