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红外和光频下的二维光谱学。

Two-dimensional spectroscopy at infrared and optical frequencies.

作者信息

Hochstrasser Robin M

机构信息

Department of Chemistry, University of Pennsylvania, Philadelphia, PA 19104-6323, USA.

出版信息

Proc Natl Acad Sci U S A. 2007 Sep 4;104(36):14190-6. doi: 10.1073/pnas.0704079104. Epub 2007 Jul 30.

Abstract

This Perspective on multidimensional spectroscopy in the optical and infrared spectral regions focuses on the principles and the scientific and technical challenges facing these new fields. The methods hold great promise for advances in the visualization of time-dependent structural changes in complex systems ranging from liquids to biological assemblies, new materials, and fundamental physical processes. The papers in this special feature on multidimensional spectroscopy in chemistry, physics, and biology are typical of many recent advances.

摘要

这篇关于光学和红外光谱区域多维光谱学的综述聚焦于这些新领域所面临的原理以及科学和技术挑战。这些方法对于推进从液体到生物组件、新材料以及基础物理过程等复杂系统中随时间变化的结构变化可视化具有巨大潜力。本期关于化学、物理和生物学多维光谱学的专题论文是众多近期进展的典型代表。

相似文献

1
Two-dimensional spectroscopy at infrared and optical frequencies.红外和光频下的二维光谱学。
Proc Natl Acad Sci U S A. 2007 Sep 4;104(36):14190-6. doi: 10.1073/pnas.0704079104. Epub 2007 Jul 30.
2
Three-dimensional structures by two-dimensional vibrational spectroscopy.二维振动光谱的三维结构。
Acc Chem Res. 2012 Nov 20;45(11):1896-905. doi: 10.1021/ar3000025. Epub 2012 Mar 29.
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Two-dimensional infrared spectroscopy: an emerging analytical tool?二维红外光谱学:一种新兴的分析工具?
Analyst. 2020 Mar 21;145(6):2014-2024. doi: 10.1039/c9an02035g. Epub 2020 Feb 13.
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Applications of two-dimensional infrared spectroscopy.二维红外光谱学的应用
Analyst. 2015 Jul 7;140(13):4336-49. doi: 10.1039/c5an00558b.

引用本文的文献

1
: Ultrafast Spectroscopy beyond the Fourier Limit Using Bayesian Inference.使用贝叶斯推理超越傅里叶极限的超快光谱学
J Phys Chem A. 2024 Oct 24;128(42):9323-9336. doi: 10.1021/acs.jpca.4c04385. Epub 2024 Oct 16.
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Atomic fluctuations in electronic materials revealed by dephasing.通过退相揭示的电子材料中的原子涨落。
Proc Natl Acad Sci U S A. 2020 Jun 2;117(22):11940-11946. doi: 10.1073/pnas.1916792117. Epub 2020 May 14.

本文引用的文献

1
Simulation of two-dimensional infrared spectroscopy of amyloid fibrils.淀粉样纤维的二维红外光谱模拟。
Proc Natl Acad Sci U S A. 2007 Sep 4;104(36):14233-6. doi: 10.1073/pnas.0700392104. Epub 2007 Aug 3.
2
Polarization-dependent optical 2D Fourier transform spectroscopy of semiconductors.半导体的偏振相关光学二维傅里叶变换光谱学。
Proc Natl Acad Sci U S A. 2007 Sep 4;104(36):14227-32. doi: 10.1073/pnas.0701273104. Epub 2007 Jul 13.
4
Transient 2D IR spectroscopy of ubiquitin unfolding dynamics.泛素解折叠动力学的瞬态二维红外光谱
Proc Natl Acad Sci U S A. 2007 Sep 4;104(36):14237-42. doi: 10.1073/pnas.0700959104. Epub 2007 Jun 5.
5
Cross-peak-specific two-dimensional electronic spectroscopy.特定交叉峰二维电子光谱学。
Proc Natl Acad Sci U S A. 2007 Sep 4;104(36):14203-8. doi: 10.1073/pnas.0701201104. Epub 2007 Jun 4.
7
Two-dimensional infrared spectroscopy detected by chirped pulse upconversion.
Opt Lett. 2007 Mar 15;32(6):713-5. doi: 10.1364/ol.32.000713.
9

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