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红外和光频下的二维光谱学。

Two-dimensional spectroscopy at infrared and optical frequencies.

作者信息

Hochstrasser Robin M

机构信息

Department of Chemistry, University of Pennsylvania, Philadelphia, PA 19104-6323, USA.

出版信息

Proc Natl Acad Sci U S A. 2007 Sep 4;104(36):14190-6. doi: 10.1073/pnas.0704079104. Epub 2007 Jul 30.

DOI:10.1073/pnas.0704079104
PMID:17664429
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC1964834/
Abstract

This Perspective on multidimensional spectroscopy in the optical and infrared spectral regions focuses on the principles and the scientific and technical challenges facing these new fields. The methods hold great promise for advances in the visualization of time-dependent structural changes in complex systems ranging from liquids to biological assemblies, new materials, and fundamental physical processes. The papers in this special feature on multidimensional spectroscopy in chemistry, physics, and biology are typical of many recent advances.

摘要

这篇关于光学和红外光谱区域多维光谱学的综述聚焦于这些新领域所面临的原理以及科学和技术挑战。这些方法对于推进从液体到生物组件、新材料以及基础物理过程等复杂系统中随时间变化的结构变化可视化具有巨大潜力。本期关于化学、物理和生物学多维光谱学的专题论文是众多近期进展的典型代表。

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Two-dimensional spectroscopy at infrared and optical frequencies.红外和光频下的二维光谱学。
Proc Natl Acad Sci U S A. 2007 Sep 4;104(36):14190-6. doi: 10.1073/pnas.0704079104. Epub 2007 Jul 30.
2
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本文引用的文献

1
Simulation of two-dimensional infrared spectroscopy of amyloid fibrils.淀粉样纤维的二维红外光谱模拟。
Proc Natl Acad Sci U S A. 2007 Sep 4;104(36):14233-6. doi: 10.1073/pnas.0700392104. Epub 2007 Aug 3.
2
Polarization-dependent optical 2D Fourier transform spectroscopy of semiconductors.半导体的偏振相关光学二维傅里叶变换光谱学。
Proc Natl Acad Sci U S A. 2007 Sep 4;104(36):14227-32. doi: 10.1073/pnas.0701273104. Epub 2007 Jul 13.
3
Hydrogen bonding and Raman, IR, and 2D-IR spectroscopy of dilute HOD in liquid D2O.重水(D₂O)中稀重水合氢离子(HOD)的氢键及拉曼光谱、红外光谱和二维红外光谱
Proc Natl Acad Sci U S A. 2007 Sep 4;104(36):14215-20. doi: 10.1073/pnas.0701482104. Epub 2007 Jun 18.
4
Transient 2D IR spectroscopy of ubiquitin unfolding dynamics.泛素解折叠动力学的瞬态二维红外光谱
Proc Natl Acad Sci U S A. 2007 Sep 4;104(36):14237-42. doi: 10.1073/pnas.0700959104. Epub 2007 Jun 5.
5
Cross-peak-specific two-dimensional electronic spectroscopy.特定交叉峰二维电子光谱学。
Proc Natl Acad Sci U S A. 2007 Sep 4;104(36):14203-8. doi: 10.1073/pnas.0701201104. Epub 2007 Jun 4.
6
Two-dimensional infrared spectral signatures of 3(10)- and alpha-helical peptides.3(10)螺旋肽和α螺旋肽的二维红外光谱特征
J Phys Chem B. 2007 Mar 29;111(12):3222-35. doi: 10.1021/jp0674874. Epub 2007 Mar 8.
7
Two-dimensional infrared spectroscopy detected by chirped pulse upconversion.
Opt Lett. 2007 Mar 15;32(6):713-5. doi: 10.1364/ol.32.000713.
8
Protein ligand migration mapped by nonequilibrium 2D-IR exchange spectroscopy.通过非平衡二维红外交换光谱法绘制蛋白质配体迁移图谱。
Proc Natl Acad Sci U S A. 2007 Sep 4;104(36):14243-8. doi: 10.1073/pnas.0607758104. Epub 2007 Jan 29.
9
Coherent control of cross-peaks in chirality-induced two-dimensional optical signals of excitons.
J Chem Phys. 2006 Dec 14;125(22):224504. doi: 10.1063/1.2397686.
10
Multidimensional infrared spectroscopy of water. I. Vibrational dynamics in two-dimensional IR line shapes.水的多维红外光谱。I. 二维红外线形中的振动动力学。
J Chem Phys. 2006 Nov 21;125(19):194521. doi: 10.1063/1.2382895.