Ganesh Nikhil, Zhang Wei, Mathias Patrick C, Chow Edmond, Soares J A N T, Malyarchuk Viktor, Smith Adam D, Cunningham Brian T
Nano Sensors Group, University of Illinois at Urbana-Champaign, 208 North Wright Street, Urbana, Illinois 61801, USA.
Nat Nanotechnol. 2007 Aug;2(8):515-20. doi: 10.1038/nnano.2007.216. Epub 2007 Jul 29.
Colloidal quantum dots display a wide range of novel optical properties that could prove useful for many applications in photonics. Here, we report the enhancement of fluorescence emission from colloidal quantum dots on the surface of two-dimensional photonic crystal slabs. The enhancement is due to a combination of high-intensity near fields and strong coherent scattering effects, which we attribute to leaky eigenmodes of the photonic crystal. By fabricating two-dimensional photonic crystal slabs that operate at visible wavelengths and engineering their leaky modes so that they overlap with the absorption and emission wavelengths of the quantum dots, we demonstrate that the fluorescence intensity can be enhanced by a factor of up to 108 compared with quantum dots on an unpatterned surface.
胶体量子点展现出一系列新颖的光学特性,这些特性在光子学的许多应用中可能会很有用。在此,我们报告了二维光子晶体平板表面上胶体量子点荧光发射的增强。这种增强是高强度近场和强相干散射效应共同作用的结果,我们将其归因于光子晶体的泄漏本征模。通过制造在可见光波长下工作的二维光子晶体平板,并设计其泄漏模使其与量子点的吸收和发射波长重叠,我们证明与无图案表面上的量子点相比,荧光强度可增强高达108倍。