Benson Eric E, Kubiak Clifford P, Sathrum Aaron J, Smieja Jonathan M
Department of Chemistry and Biochemistry, University of California San Diego, 9500 Gilman Drive MC 0358, La Jolla, CA 92093, USA.
Chem Soc Rev. 2009 Jan;38(1):89-99. doi: 10.1039/b804323j. Epub 2008 Oct 24.
Research in the field of catalytic reduction of carbon dioxide to liquid fuels has grown rapidly in the past few decades. This is due to the increasing amount of carbon dioxide in the atmosphere and a steady climb in global fuel demand. This tutorial review will present much of the significant work that has been done in the field of electrocatalytic and homogeneous reduction of carbon dioxide over the past three decades. It will then extend the discussion to the important conclusions from previous work and recommendations for future directions to develop a catalytic system that will convert carbon dioxide to liquid fuels with high efficiencies.
在过去几十年中，将二氧化碳催化还原为液体燃料领域的研究迅速发展。这是由于大气中二氧化碳含量不断增加以及全球燃料需求稳步攀升。本教程综述将介绍过去三十年来在二氧化碳电催化和均相还原领域所做的许多重要工作。然后，将讨论扩展到先前工作得出的重要结论以及未来发展高效将二氧化碳转化为液体燃料的催化系统方向的建议。
