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亚稳态暗态使具有衍射极限分辨率的钻石中的氮空位中心的基态损耗显微镜成为可能。

Metastable dark States enable ground state depletion microscopy of nitrogen vacancy centers in diamond with diffraction-unlimited resolution.

机构信息

Department of NanoBiophotonics, Max Planck Institute for Biophysical Chemistry, Am Fassberg 11, 37077 Gottingen, Germany.

出版信息

Nano Lett. 2010 Aug 11;10(8):3199-203. doi: 10.1021/nl102156m.

Abstract

Current far-field optical nanoscopy schemes overcome the diffraction barrier by ensuring that adjacent features assume different states upon detection. Ideally, the transition between these states can be repeated endlessly and, if performed optically, with low levels of light. Here we report such optical switching, realized by pairing the luminescent triplet and a long-lived dark state of diamond color centers, enabling their imaging with a resolution >10 times beyond the diffraction barrier (<20 nm).

摘要

当前的远场光学纳米显微镜方案通过确保相邻特征在检测时呈现不同状态来克服衍射障碍。理想情况下,这些状态之间的转换可以无休止地重复,如果是通过光学方式实现的,则可以以低水平的光进行。在这里,我们报告了这种光学切换,通过将发光三重态和钻石色心的长寿命暗态配对来实现,从而能够以超过衍射障碍 (>20nm) 的分辨率 (>10 倍) 对其进行成像。

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