Chang Yuan-Ming, Jian Sheng-Rui, Juang Jenh-Yih
Nanoscale Res Lett. 2010 Jun 8;5(9):1456-1463. doi: 10.1007/s11671-010-9661-7.
A lithography-free method for fabricating the nanogrids and quasi-beehive nanostructures on Si substrates is developed. It combines sequential treatments of thermal annealing with reactive ion etching (RIE) on SiGe thin films grown on (100)-Si substrates. The SiGe thin films deposited by ultrahigh vacuum chemical vapor deposition form self-assembled nanoislands via the strain-induced surface roughening (Asaro-Tiller-Grinfeld instability) during thermal annealing, which, in turn, serve as patterned sacrifice regions for subsequent RIE process carried out for fabricating nanogrids and beehive-like nanostructures on Si substrates. The scanning electron microscopy and atomic force microscopy observations confirmed that the resultant pattern of the obtained structures can be manipulated by tuning the treatment conditions, suggesting an interesting alternative route of producing self-organized nanostructures.
开发了一种在硅衬底上制造纳米网格和准蜂巢状纳米结构的无光刻方法。它将热退火的顺序处理与在(100)-硅衬底上生长的硅锗薄膜上的反应离子蚀刻(RIE)相结合。通过超高真空化学气相沉积沉积的硅锗薄膜在热退火过程中通过应变诱导的表面粗糙度(阿萨罗-蒂勒-格林菲尔德不稳定性)形成自组装纳米岛,这些纳米岛反过来又作为图案化的牺牲区域,用于随后在硅衬底上制造纳米网格和蜂巢状纳米结构的反应离子蚀刻工艺。扫描电子显微镜和原子力显微镜观察证实,所得结构的最终图案可以通过调整处理条件来控制,这表明了一种生产自组织纳米结构的有趣替代途径。