JILA, National Institute of Standards and Technology and University of Colorado, Boulder, Colorado 80309-0440, USA.
Phys Rev Lett. 2010 Jun 18;104(24):247401. doi: 10.1103/PhysRevLett.104.247401. Epub 2010 Jun 15.
Detailed electronic many-body configurations are extracted from quantitatively measured time-resolved nonlinear absorption spectra of resonantly excited GaAs quantum wells. The microscopic theory assigns the observed spectral changes to a unique mixture of electron-hole plasma, exciton, and polarization effects. Strong transient gain is observed only under cocircular pump-probe conditions and is attributed to the transfer of pump-induced coherences to the probe.
从定量测量的共振激发 GaAs 量子阱的时间分辨非线性吸收光谱中提取出详细的电子多体构型。微观理论将观察到的光谱变化归因于电子-空穴等离子体、激子和极化效应的独特混合。只有在共圆泵浦-探测条件下才观察到强瞬态增益,这归因于泵浦诱导的相干态向探测的转移。