Department of Biochemistry, Biophysics and Molecular Biology, Iowa State University, Ames, IA 50011, USA.
Appl Environ Microbiol. 2011 Sep;77(18):6441-50. doi: 10.1128/AEM.05358-11. Epub 2011 Jul 29.
Escherichia coli K-12 strain MG1655 was engineered to coproduce acetaldehyde and hydrogen during glucose fermentation by the use of exogenous acetyl-coenzyme A (acetyl-CoA) reductase (for the conversion of acetyl-CoA to acetaldehyde) and the native formate hydrogen lyase. A putative acetaldehyde dehydrogenase/acetyl-CoA reductase from Salmonella enterica (SeEutE) was cloned, produced at high levels, and purified by nickel affinity chromatography. In vitro assays showed that this enzyme had both acetaldehyde dehydrogenase activity (68.07 ± 1.63 μmol min(-1) mg(-1)) and the desired acetyl-CoA reductase activity (49.23 ± 2.88 μmol min(-1) mg(-1)). The eutE gene was engineered into an E. coli mutant lacking native glucose fermentation pathways (ΔadhE, ΔackA-pta, ΔldhA, and ΔfrdC). The engineered strain (ZH88) produced 4.91 ± 0.29 mM acetaldehyde while consuming 11.05 mM glucose but also produced 6.44 ± 0.26 mM ethanol. Studies showed that ethanol was produced by an unknown alcohol dehydrogenase(s) that converted the acetaldehyde produced by SeEutE to ethanol. Allyl alcohol was used to select for mutants with reduced alcohol dehydrogenase activity. Three allyl alcohol-resistant mutants were isolated; all produced more acetaldehyde and less ethanol than ZH88. It was also found that modifying the growth medium by adding 1 g of yeast extract/liter and lowering the pH to 6.0 further increased the coproduction of acetaldehyde and hydrogen. Under optimal conditions, strain ZH136 converted glucose to acetaldehyde and hydrogen in a 1:1 ratio with a specific acetaldehyde production rate of 0.68 ± 0.20 g h(-1) g(-1) dry cell weight and at 86% of the maximum theoretical yield. This specific production rate is the highest reported thus far and is promising for industrial application. The possibility of a more efficient "no-distill" ethanol fermentation procedure based on the coproduction of acetaldehyde and hydrogen is discussed.
将大肠杆菌 K-12 菌株 MG1655 工程改造为在葡萄糖发酵过程中同时产生乙醛和氢气,方法是使用外源性乙酰辅酶 A(乙酰辅酶 A)还原酶(将乙酰辅酶 A 转化为乙醛)和天然甲酸氢裂解酶。从沙门氏菌中克隆、高水平表达并通过镍亲和层析纯化了一种假定的乙醛脱氢酶/乙酰辅酶 A 还原酶(SeEutE)。体外测定表明,该酶具有乙醛脱氢酶活性(68.07±1.63μmol min-1mg-1)和所需的乙酰辅酶 A 还原酶活性(49.23±2.88μmol min-1mg-1)。将 eutE 基因工程改造到缺乏天然葡萄糖发酵途径的大肠杆菌突变体(ΔadhE、ΔackA-pta、ΔldhA 和 ΔfrdC)中。工程菌株(ZH88)产生 4.91±0.29mM 乙醛,同时消耗 11.05mM 葡萄糖,但也产生 6.44±0.26mM 乙醇。研究表明,乙醇是由一种未知的醇脱氢酶(s)产生的,该酶将 SeEutE 产生的乙醛转化为乙醇。使用烯丙醇选择具有降低的醇脱氢酶活性的突变体。分离出三个烯丙醇抗性突变体;与 ZH88 相比,它们都产生了更多的乙醛和更少的乙醇。还发现,通过添加 1g/L 酵母提取物和将 pH 值降低至 6.0 来修饰生长培养基,进一步增加了乙醛和氢气的共生产。在最佳条件下,菌株 ZH136 将葡萄糖转化为乙醛和氢气,比例为 1:1,比产率为 0.68±0.20g h-1g-1 干细胞重量,达到最大理论产率的 86%。这个比产率是迄今为止报道的最高值,有望在工业应用中得到应用。讨论了基于乙醛和氢气共生产的更有效的“无蒸馏”乙醇发酵工艺的可能性。