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等离子体吸收器中金纳米颗粒的光热重塑

Photothermal reshaping of gold nanoparticles in a plasmonic absorber.

作者信息

Wang Jing, Chen Yiting, Chen Xi, Hao Jiaming, Yan Min, Qiu Min

机构信息

Division of Optics and Photonics, Royal Institute of Technology, KTH, Electrum 229, 164 40 Kista, Sweden.

出版信息

Opt Express. 2011 Jul 18;19(15):14726-34. doi: 10.1364/OE.19.014726.

Abstract

We experimentally demonstrate that a metamaterial nanostructure can have a localized heating response owing to plasmonic resonances in the near-infrared wavelength range (from 1.5 to 2 µm). With a broadband nanosecond-pulse light, the temperature of composing gold particles in the nanostructure can be easily increased to over 900K within only several nanoseconds, resulting in re-shaping of the particles. The photothermal effect is elaborated with finite-element based numerical simulations. The absorption resonance can in principle be tailored with a great freedom by choosing appropriate metamaterial parameters. The light-induced heating in an artificial metamaterial can be potentially used for all-optical acute temperature tuning in a micro-environment, which may open new frontiers especially in nanotechnology and biotechnology.

摘要

我们通过实验证明,超材料纳米结构在近红外波长范围(1.5至2微米)内由于等离子体共振可产生局部加热响应。使用宽带纳秒脉冲光,纳米结构中构成金颗粒的温度可在仅几纳秒内轻松升高至900K以上,导致颗粒重新塑形。通过基于有限元的数值模拟阐述了光热效应。原则上,通过选择合适的超材料参数,可以非常自由地调整吸收共振。人工超材料中的光致加热可潜在地用于微环境中的全光急性温度调节,这可能尤其在纳米技术和生物技术领域开辟新的前沿。

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