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石墨烯-SiO₂界面狄拉克等离激元的红外纳米光谱学

Infrared nanoscopy of dirac plasmons at the graphene-SiO₂ interface.

机构信息

Department of Physics, University of California San Diego, La Jolla, California 92093, United States.

出版信息

Nano Lett. 2011 Nov 9;11(11):4701-5. doi: 10.1021/nl202362d. Epub 2011 Oct 12.

DOI:10.1021/nl202362d
PMID:21972938
Abstract

We report on infrared (IR) nanoscopy of 2D plasmon excitations of Dirac fermions in graphene. This is achieved by confining mid-IR radiation at the apex of a nanoscale tip: an approach yielding 2 orders of magnitude increase in the value of in-plane component of incident wavevector q compared to free space propagation. At these high wavevectors, the Dirac plasmon is found to dramatically enhance the near-field interaction with mid-IR surface phonons of SiO(2) substrate. Our data augmented by detailed modeling establish graphene as a new medium supporting plasmonic effects that can be controlled by gate voltage.

摘要

我们报告了在狄拉克费米子的二维等离激元激发的中红外(IR)纳米光谱学。这是通过将中红外辐射限制在纳米级尖端的顶点来实现的:与自由空间传播相比,这种方法使入射波矢 q 的平面分量的值增加了两个数量级。在这些高波矢下,发现狄拉克等离激元极大地增强了与 SiO2 衬底的中红外表面声子的近场相互作用。我们的数据通过详细的建模得到了增强,确定了石墨烯作为一种新的支持等离子体效应的介质,该效应可以通过栅极电压来控制。

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