Max Planck Institute for the Science of Light, D-91058 Erlangen, Germany.
Phys Rev Lett. 2012 Jun 8;108(23):233001. doi: 10.1103/PhysRevLett.108.233001.
We devise new optical antennas that reduce the excited-state radiative lifetimes of emitters to the order of 100 fs while maintaining quantum efficiencies of about 80% at a broadband operation. Here, we combine metallic nanoparticles with planar dielectric structures and exploit design strategies from plasmonic nanoantennas and concepts from cavity quantum electrodynamics to maximize the local density of states and minimize the nonradiative losses incurred by the metallic constituents. The proposed metallodielectric hybrid antennas promise an important impact on various fundamental and applied research fields, including photophysics, ultrafast plasmonics, bright single-photon sources, and Raman spectroscopy.
我们设计了新的光学天线,可将发射器的激发态辐射寿命降低到 100fs 左右,同时在宽带操作下保持约 80%的量子效率。在这里,我们将金属纳米粒子与平面介电结构相结合,并利用等离子体纳米天线的设计策略和腔量子电动力学的概念,最大限度地提高局部态密度并最小化金属成分引起的非辐射损耗。所提出的金属-介质混合天线有望对各种基础研究和应用研究领域产生重要影响,包括光物理、超快等离子体学、亮单光子源和拉曼光谱学。