Institut de Physique et Chimie des Matériaux de Strasbourg, Université de Strasbourg, CNRS UMR 7504, 23 rue du Loess, BP 43, F-67034 Strasbourg Cedex 2, France.
Phys Rev Lett. 2013 Mar 8;110(10):106801. doi: 10.1103/PhysRevLett.110.106801. Epub 2013 Mar 5.
We consider a two-dimensional honeycomb lattice of metallic nanoparticles, each supporting a localized surface plasmon, and study the quantum properties of the collective plasmons resulting from the near-field dipolar interaction between the nanoparticles. We analytically investigate the dispersion, the effective Hamiltonian, and the eigenstates of the collective plasmons for an arbitrary orientation of the individual dipole moments. When the polarization points close to the normal to the plane, the spectrum presents Dirac cones, similar to those present in the electronic band structure of graphene. We derive the effective Dirac Hamiltonian for the collective plasmons and show that the corresponding spinor eigenstates represent Dirac-like massless bosonic excitations that present similar effects to electrons in graphene, such as a nontrivial Berry phase and the absence of backscattering off smooth inhomogeneities. We further discuss how one can manipulate the Dirac points in the Brillouin zone and open a gap in the collective plasmon dispersion by modifying the polarization of the localized surface plasmons, paving the way for a fully tunable plasmonic analogue of graphene.
我们考虑一个二维的金属纳米粒子蜂窝晶格,每个纳米粒子都支持局域表面等离激元,并研究了由纳米粒子之间的近场偶极相互作用产生的集体等离激元的量子性质。我们分析研究了集体等离激元的色散、有效哈密顿量和本征态,对于任意的单个偶极矩取向。当极化方向接近平面的法向时,谱呈现出狄拉克锥,类似于石墨烯中的电子能带结构中的狄拉克锥。我们推导出了集体等离激元的有效狄拉克哈密顿量,并表明相应的旋量本征态代表了类似狄拉克的无质量玻色激发,它们在石墨烯中的电子具有类似的效应,例如非平凡的贝里相位和对光滑非均匀性的无背散射。我们进一步讨论了如何通过改变局域表面等离激元的极化来操纵狄拉克点和在集体等离激元色散中打开能隙,为完全可调谐的石墨烯等离子体类似物铺平了道路。