Center for Nanophotonics, FOM Institute AMOLF, Science Park 104, 1098 XG Amsterdam, The Netherlands.
Phys Rev Lett. 2013 May 24;110(21):217405. doi: 10.1103/PhysRevLett.110.217405. Epub 2013 May 23.
We experimentally demonstrate control of the rate of spontaneous emission in a tunable hybrid photonic system that consists of two canonical building blocks for spontaneous emission control, an optical antenna and a mirror, each providing a modification of the local density of optical states (LDOS). We couple fluorophores to a plasmonic antenna to create a superemitter with an enhanced decay rate. In a superemitter analog of the seminal Drexhage experiment we probe the LDOS of a nanomechanically approached mirror. Because of the electrodynamic interaction of the antenna with its own mirror image, the superemitter traces the inverse of the LDOS enhancement provided by the mirror, in stark contrast to a bare source, whose decay rate is proportional to the mirror LDOS.
我们通过实验演示了在可调谐混合光子系统中对自发辐射速率的控制,该系统由两个自发辐射控制的典型构建块组成,分别是光学天线和反射镜,它们各自对局部光态密度(LDOS)进行了修正。我们将荧光团耦合到等离子体天线上,以创建具有增强衰减率的超强发射器。在对开创性的 Drexhage 实验的超强发射器模拟中,我们探测了纳米机械接近的反射镜的 LDOS。由于天线与其自身镜像的电动力学相互作用,超强发射器跟踪反射镜提供的 LDOS 增强的逆,这与裸光源形成鲜明对比,裸光源的衰减率与反射镜的 LDOS 成正比。