Department of Condensed Matter Physics and Materials Science, Brookhaven National Laboratory, Upton, New York 11973, USA.
Nat Mater. 2013 Nov;12(11):1019-23. doi: 10.1038/nmat3723. Epub 2013 Aug 4.
One of the most intensely studied scenarios of high-temperature superconductivity (HTS) postulates pairing by exchange of magnetic excitations. Indeed, such excitations have been observed up to optimal doping in the cuprates. In the heavily overdoped regime, neutron scattering measurements indicate that magnetic excitations have effectively disappeared, and this has been argued to cause the demise of HTS with overdoping. Here we use resonant inelastic X-ray scattering, which is sensitive to complementary parts of reciprocal space, to measure the evolution of the magnetic excitations in La(2-x)Sr(x)CuO4 across the entire phase diagram, from a strongly correlated insulator (x = 0) to a non-superconducting metal (x = 0.40). For x = 0, well-defined magnon excitations are observed. These magnons broaden with doping, but they persist with a similar dispersion and comparable intensity all the way to the non-superconducting, heavily overdoped metallic phase. The destruction of HTS with overdoping is therefore caused neither by the general disappearance nor by the overall softening of magnetic excitations. Other factors, such as the redistribution of spectral weight, must be considered.
高温超导(HTS)的一个研究热点是通过磁激子交换来实现配对。事实上,在铜酸盐的最佳掺杂范围内已经观察到了这种激子。在过掺杂区域,中子散射测量表明磁激子已经有效消失,这被认为是过掺杂导致 HTS 消失的原因。在这里,我们使用共振非弹性 X 射线散射,它对倒易空间的互补部分敏感,来测量 La(2-x)Sr(x)CuO4 中的磁激子在整个相图中的演化,从强关联绝缘体(x = 0)到非超导金属(x = 0.40)。对于 x = 0,我们观察到了定义明确的磁振子激发。这些磁振子随着掺杂而展宽,但它们一直保持着相似的色散和相当的强度,直到非超导的过掺杂金属相。因此,过掺杂导致 HTS 破坏的原因不是磁激子的普遍消失或整体软化。必须考虑其他因素,如光谱权重的重新分配。