Hu Shishan, Paulson Suzanne E, Fruin Scott, Kozawa Kathleen, Mara Steve, Winer Arthur M
California Air Resources Board, Monitoring and Laboratory Division, 9528 Telstar Ave, El Monte, CA 91731 ; Environmental Health Sciences Department, School of Public Health, 650 Charles E. Young Drive South, University of California, Los Angeles, CA 90095-1772 ; Department of Atmospheric and Oceanic Sciences, 405 Hilgard Ave., University of California, Los Angeles, CA 90095-1565.
Atmos Environ (1994). 2012 May 1;51:311-319. doi: 10.1016/j.atmosenv.2011.12.055.
We observed elevated air pollutant concentrations, especially of ultrafine particles (UFP), black carbon (BC) and NO, across the residential neighborhood of the Boyle Heights Community (BH) of Los Angeles, California. Using an electric vehicle mobile platform equipped with fast response instruments, real-time air pollutant concentrations were measured in BH in spring and summer of 2008. Pollutant concentrations varied significantly in the two seasons, on different days, and by time of day, with an overall average UFP concentration in the residential areas of ~33 000 cm. The averaged UFP, BC, and NO concentrations measured on Soto St, a major surface street in BH, were 57 000 cm, 5.1 µg m, and 67 ppb, respectively. Concentrations of UFP across the residential areas in BH were nearly uniform spatially, in contrast to other areas in the greater metropolitan area of Los Angeles where UFP concentrations exhibit strong gradients downwind of roadways. We attribute this "UFP cloud" to high traffic volumes, including heavy duty diesel trucks on the freeways which surround and traverse BH, and substantial numbers of high-emitting vehicles (HEVs) on the surface streets traversing BH. Additionally, the high density of stop signs and lights and short block lengths, requiring frequent accelerations of vehicles, may contribute. The data also support a role for photochemical production of UFP in the afternoon. UFP concentration peaks (5 s average) of up to 9 million particles cm were also observed immediately behind HEVs when they accelerated from stop lights in the BH neighborhood and areas immediately adjacent. Although encounters with HEV during mornings accounted for only about 6% and 17% of time spent monitoring residential areas and major surface streets, HEV contributed to about 28% and 53% of total ultrafine particles measured on the route, respectively. The observation of elevated pollutant number concentrations across the Boyle Heights community highlights how multiple factors combine to create high pollutant levels, and has important human exposure assessment implications, including the potential utility of our data as inputs to epidemiological studies.
我们观察到加利福尼亚州洛杉矶市博伊尔高地社区(BH)居民区的空气污染物浓度升高,尤其是超细颗粒物(UFP)、黑碳(BC)和一氧化氮(NO)。使用配备快速响应仪器的电动汽车移动平台,于2008年春季和夏季在BH测量了实时空气污染物浓度。两个季节、不同日期以及一天中的不同时段,污染物浓度差异显著,居民区的UFP总体平均浓度约为每立方厘米33000个。在BH的一条主要地面街道索托街测量的UFP、BC和NO平均浓度分别为每立方厘米57000个、每立方米5.1微克和67 ppb。与洛杉矶大都市区的其他区域不同,BH居民区的UFP浓度在空间上几乎是均匀的,在其他区域,UFP浓度在道路下风方向呈现出强烈的梯度变化。我们将这种“UFP云”归因于高交通流量,包括环绕并穿过BH的高速公路上的重型柴油卡车,以及穿过BH的地面街道上大量的高排放车辆(HEV)。此外,停车标志和信号灯的高密度以及街区长度较短,导致车辆频繁加速,这可能也起到了一定作用。数据还支持下午UFP的光化学生成作用。当HEV在BH社区及紧邻区域从停车信号灯处加速时,在其后方还立即观察到UFP浓度峰值(5秒平均值)高达每立方厘米900万个颗粒。尽管早晨遇到HEV的时间仅分别占监测居民区和主要地面街道时间的约6%和17%,但HEV分别贡献了该路线上测量的总超细颗粒物的约28%和53%。博伊尔高地社区污染物数量浓度升高的观察结果凸显了多种因素如何共同导致高污染物水平,并且对人体暴露评估具有重要意义,包括我们的数据作为流行病学研究输入的潜在效用。