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室内灰尘和多表面灰尘中邻苯二甲酸酯浓度与日本住宅内部材料的关联。

Associations of phthalate concentrations in floor dust and multi-surface dust with the interior materials in Japanese dwellings.

机构信息

Hokkaido University Graduate School of Medicine, Department of Public Health Sciences, Kita 15, Nishi 7, Kita-ku, Sapporo 060-8638, Japan.

出版信息

Sci Total Environ. 2014 Jan 15;468-469:147-57. doi: 10.1016/j.scitotenv.2013.07.107. Epub 2013 Sep 4.

Abstract

Phthalates are widely used as plasticizers in numerous products. However, there has been some concern about the various effects they may have on human health. Thus, household phthalate levels are an important public health issue. While many studies have assessed phthalate levels in house dust, the association of these levels with building characteristics has scarcely been examined. The present study investigated phthalate levels in house dust samples collected from the living areas of homes, and examined associations between these phthalate levels and the interior materials. Dust was collected from two portions of the living area: floor dust from the entire floor surface, and multi-surface dust from objects more than 35 cm above the floor. The levels of seven phthalates were measured using gas chromatography/mass spectrometry in selective ion monitoring mode. Phthalate levels were higher in multi-surface dust than in floor dust. Among floor dust samples, those from dwellings with compressed wooden flooring had significantly higher levels of di-iso-butyl phthalate compared to those with other floor materials, while polyvinyl chloride (PVC) flooring was associated with higher di-2-ethylhexyl phthalate (DEHP) levels. Among multi-surface dust samples, higher levels of DEHP and di-iso-nonyl phthalate (DINP) were found in samples from homes with PVC wallpaper than without. The number of PVC interior materials was significantly positively correlated with the levels of DEHP and DINP in multi-surface dust. The phthalate levels in multi-surface dust were associated with the interior surface materials, and those in floor dust were directly related to the flooring materials. Our findings show that when using house dust as an exposure assessment, it is very important to note where the samples were collected from. The present report provides useful information about the association between phthalates and dust inside dwellings, which will assist with establishing public health provisions.

摘要

邻苯二甲酸酯作为增塑剂被广泛应用于各种产品中。然而,人们对其对人类健康可能产生的各种影响存在一些担忧。因此,家庭环境中的邻苯二甲酸酯水平是一个重要的公共卫生问题。虽然许多研究都评估了房屋灰尘中的邻苯二甲酸酯水平,但这些水平与建筑物特征之间的关系却很少被研究过。本研究调查了从家庭居住区域采集的房屋灰尘样本中的邻苯二甲酸酯水平,并研究了这些邻苯二甲酸酯水平与室内材料之间的关系。灰尘分别从居住区域的两个部分采集:整个地板表面的地板灰尘,以及超过地板 35 厘米以上物体的多表面灰尘。使用气相色谱/质谱联用仪在选择离子监测模式下测量了七种邻苯二甲酸酯的水平。多表面灰尘中的邻苯二甲酸酯水平高于地板灰尘。在地板灰尘样本中,与其他地板材料相比,压缩木地板住宅中的邻苯二甲酸二异丁酯水平明显较高,而聚氯乙烯(PVC)地板与较高的邻苯二甲酸二(2-乙基己基)酯(DEHP)水平相关。在多表面灰尘样本中,发现含有 PVC 壁纸的住宅样本中的邻苯二甲酸二异壬酯(DINP)和 DEHP 水平较高。家中 PVC 内饰材料的数量与多表面灰尘中的 DEHP 和 DINP 水平呈显著正相关。多表面灰尘中的邻苯二甲酸酯水平与室内表面材料有关,地板灰尘中的邻苯二甲酸酯水平则与地板材料直接相关。我们的研究结果表明,当使用房屋灰尘作为暴露评估时,非常重要的是要注意采样的位置。本报告提供了有关房屋内邻苯二甲酸酯与灰尘之间关系的有用信息,这将有助于制定公共卫生规定。

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