Laboratory for Aviation and the Environment, Massachusetts Institute of Technology , 77 Massachusetts Avenue, Cambridge, Massachusetts 02139, United States.
Environ Sci Technol. 2013;47(21):12557-65. doi: 10.1021/es4030782. Epub 2013 Oct 10.
Middle distillate (MD) transportation fuels, including diesel and jet fuel, make up almost 30% of liquid fuel consumption in the United States. Alternative drop-in MD and biodiesel could potentially reduce dependence on crude oil and the greenhouse gas intensity of transportation. However, the water and land resource requirements of these novel fuel production technologies must be better understood. This analysis quantifies the lifecycle green and blue water consumption footprints of producing: MD from conventional crude oil; Fischer-Tropsch MD from natural gas and coal; fermentation and advanced fermentation MD from biomass; and hydroprocessed esters and fatty acids MD and biodiesel from oilseed crops, throughout the contiguous United States. We find that FT MD and alternative MD derived from rainfed biomass have lifecycle blue water consumption footprints of 1.6 to 20.1 Lwater/LMD, comparable to conventional MD, which ranges between 4.1 and 7.4 Lwater/LMD. Alternative MD derived from irrigated biomass has a lifecycle blue water consumption footprint potentially several orders of magnitude larger, between 2.7 and 22 600 Lwater/LMD. Alternative MD derived from biomass has a lifecycle green water consumption footprint between 1.1 and 19 200 Lwater/LMD. Results are disaggregated to characterize the relationship between geo-spatial location and lifecycle water consumption footprint. We also quantify the trade-offs between blue water consumption footprint and areal MD productivity, which ranges from 490 to 4200 LMD/ha, under assumptions of rainfed and irrigated biomass cultivation. Finally, we show that if biomass cultivation for alternative MD is irrigated, the ratio of the increase in areal MD productivity to the increase in blue water consumption footprint is a function of geo-spatial location and feedstock-to-fuel production pathway.
中间馏分(MD)运输燃料,包括柴油和喷气燃料,占美国液体燃料消耗的近 30%。替代的调入 MD 和生物柴油可能会减少对原油的依赖,并降低交通运输的温室气体强度。然而,这些新型燃料生产技术的水和土地资源需求必须得到更好的理解。本分析量化了在美国本土生产以下产品的生命周期绿水和蓝水消耗足迹:从常规原油中提取 MD;从天然气和煤中提取费托 MD;从生物质中发酵和先进发酵提取 MD;以及从油籽作物中提取氢化酯和脂肪酸 MD 和生物柴油。我们发现,FT MD 和雨养生物质衍生的替代 MD 的生命周期蓝水消耗足迹为 1.6 至 20.1 Lwater/LMD,与常规 MD(4.1 至 7.4 Lwater/LMD)相当。灌溉生物质衍生的替代 MD 的生命周期蓝水消耗足迹可能大几个数量级,为 2.7 至 22600 Lwater/LMD。生物质衍生的替代 MD 的生命周期绿水消耗足迹为 1.1 至 19200 Lwater/LMD。结果按地理位置进行细分,以描述地理位置与生命周期水消耗足迹之间的关系。我们还量化了在雨养和灌溉生物质种植假设下,蓝水消耗足迹与 MD 单位面积生产力之间的权衡关系,范围从 490 至 4200 LMD/ha。最后,我们表明,如果替代 MD 的生物质种植是灌溉的,那么单位面积 MD 生产力的增加与蓝水消耗足迹的增加之比是地理位置和原料到燃料生产途径的函数。