Nonlinear Physics Centre, Research School of Physics and Engineering, The Australian National University , Canberra ACT 0200, Australia.
ACS Nano. 2013 Sep 24;7(9):7824-32. doi: 10.1021/nn402736f. Epub 2013 Aug 21.
Interference of optically induced electric and magnetic modes in high-index all-dielectric nanoparticles offers unique opportunities for tailoring directional scattering and engineering the flow of light. In this article we demonstrate theoretically and experimentally that the interference of electric and magnetic optically induced modes in individual subwavelength silicon nanodisks can lead to the suppression of resonant backscattering and to enhanced resonant forward scattering of light. To this end we spectrally tune the nanodisk's fundamental electric and magnetic resonances with respect to each other by a variation of the nanodisk aspect ratio. This ability to tune two modes of different character within the same nanoparticle provides direct control over their interference, and, in consequence, allows for engineering the particle's resonant and off-resonant scattering patterns. Most importantly, measured and numerically calculated transmittance spectra reveal that backward scattering can be suppressed and forward scattering can be enhanced at resonance for the particular case of overlapping electric and magnetic resonances. Our experimental results are in good agreement with calculations based on the discrete dipole approach as well as finite-integral frequency-domain simulations. Furthermore, we show useful applications of silicon nanodisks with tailored resonances as optical nanoantennas with strong unidirectional emission from a dipole source.
高折射率全介质纳米粒子中光诱导的电和磁模式的干涉为定向散射的调整和光流工程提供了独特的机会。在本文中,我们从理论和实验上证明,单个亚波长硅纳米盘的电和磁光诱导模式的干涉可以导致共振后向散射的抑制和光的共振前向散射的增强。为此,我们通过改变纳米盘的纵横比来实现纳米盘的基本电和磁共振之间的光谱调谐。在同一纳米粒子中调谐两种不同特性的模式的这种能力提供了对它们干涉的直接控制,并且,因此,允许对粒子的共振和非共振散射模式进行工程设计。最重要的是,测量和数值计算的透射光谱表明,对于电和磁共振重叠的特殊情况,可以抑制后向散射并增强共振时的前向散射。我们的实验结果与基于离散偶极子方法以及有限积分频域模拟的计算结果吻合良好。此外,我们展示了具有定制共振的硅纳米盘作为光学纳米天线的有用应用,其具有从偶极子源的强单向发射。