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石墨烯的相分辨表面等离子体干涉测量。

Phase-resolved surface plasmon interferometry of graphene.

机构信息

Department of Physics, Department of Chemistry, and JILA, University of Colorado, Boulder, Colorado 80309, USA.

出版信息

Phys Rev Lett. 2014 Aug 1;113(5):055502. doi: 10.1103/PhysRevLett.113.055502. Epub 2014 Jul 30.

Abstract

The surface plasmon polaritons (SPPs) of graphene reflect the microscopic spatial variations of underlying electronic structure and dynamics. Here, we excite and image the graphene SPP response in phase and amplitude by near-field interferometry. We develop an analytic cavity model that can self-consistently describe the SPP response function for edge, grain boundary, and defect SPP reflection and scattering. The derived SPP wave vector, damping, and carrier mobility agree with the results from more complex models. Spatial variations in the Fermi level and associated variations in dopant concentration reveal a nanoscale spatial inhomogeneity in the reduced conductivity at internal boundaries. The additional SPP phase information thus opens a new degree of freedom for spatial and spectral graphene SPP tuning and modulation for optoelectronics applications.

摘要

石墨烯的表面等离激元(SPPs)反映了其底层电子结构和动力学的微观空间变化。在这里,我们通过近场干涉测量法激发并以相位和幅度成像石墨烯 SPP 的响应。我们开发了一个解析腔模型,该模型可以自洽地描述边缘、晶界和缺陷 SPP 反射和散射的 SPP 响应函数。所得到的 SPP 波矢、阻尼和载流子迁移率与更复杂模型的结果一致。费米能级的空间变化以及相关的掺杂浓度变化揭示了内部边界处的电导率降低的纳米级空间非均匀性。因此,额外的 SPP 相位信息为空间和光谱石墨烯 SPP 的调谐和调制开辟了一个新的自由度,可用于光电应用。

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