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在共振非弹性软X射线散射中对散射辐射的能量和线性极化进行同步测量。

The simultaneous measurement of energy and linear polarization of the scattered radiation in resonant inelastic soft x-ray scattering.

作者信息

Braicovich L, Minola M, Dellea G, Le Tacon M, Moretti Sala M, Morawe C, Peffen J-Ch, Supruangnet R, Yakhou F, Ghiringhelli G, Brookes N B

机构信息

CNR-SPIN and Dipartimento di Fisica, Politecnico di Milano, piazza Leonardo Da Vinci 32, Milano I-20133, Italy.

Max-Planck-Institut für Festkörperforschung, Heisenbergstrasse 1, D-70569 Stuttgart, Germany.

出版信息

Rev Sci Instrum. 2014 Nov;85(11):115104. doi: 10.1063/1.4900959.

Abstract

Resonant Inelastic X-ray Scattering (RIXS) in the soft x-ray range is an element-specific energy-loss spectroscopy used to probe the electronic and magnetic excitations in strongly correlated solids. In the recent years, RIXS has been progressing very quickly in terms of energy resolution and understanding of the experimental results, but the interpretation of spectra could further improve, sometimes decisively, from a full knowledge of the polarization of incident and scattered photons. Here we present the first implementation, in a high resolution soft-RIXS spectrometer used to analyze the scattered radiation, of a device allowing the measurement of the degree of linear polarization. The system, based on a graded W/B4C multilayer mirror installed in proximity of the CCD detector, has been installed on the AXES spectrometer at the ESRF (European Synchrotron Radiation Facility); it has been fully characterized and it has been used for a demonstration experiment at the Cu L3 edge on a high-Tc superconducting cuprate. The loss in efficiency suffered by the spectrometer equipped with this test facility was a factor 17.5. We propose also a more advanced version, suitable for a routine use on the next generation of RIXS spectrometers and with an overall efficiency up to 10%.

摘要

软X射线范围内的共振非弹性X射线散射(RIXS)是一种元素特异性能量损失光谱,用于探测强关联固体中的电子和磁激发。近年来,RIXS在能量分辨率和对实验结果的理解方面进展非常迅速,但从对入射光子和散射光子极化的全面了解来看,光谱的解释有时仍可决定性地进一步改进。本文展示了在用于分析散射辐射的高分辨率软X射线RIXS光谱仪中首次实现的一种能够测量线性极化度的装置。该系统基于安装在电荷耦合器件(CCD)探测器附近的渐变W/B4C多层镜,已安装在欧洲同步辐射装置(ESRF)的AXES光谱仪上;它已得到充分表征,并已用于在高温超导铜酸盐的铜L3边缘进行的演示实验中。配备此测试装置的光谱仪效率损失为17.5倍。我们还提出了一个更先进的版本,适用于下一代RIXS光谱仪的常规使用,总体效率高达10%。

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