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美国特拉华州不同室内环境中地板灰尘邻苯二甲酸盐的比较、关联及风险评估。

Comparison, association, and risk assessment of phthalates in floor dust at different indoor environments in Delaware, USA.

作者信息

Bi Xiaolong, Yuan Shoujun, Pan Xiaojun, Winstead Cherese, Wang Qiquan

机构信息

a Chemistry Department , Delaware State University , Dover , Delaware , USA.

b School of Energy and Power Engineering , Nanjing Institute of Technology , Jiangsu , China.

出版信息

J Environ Sci Health A Tox Hazard Subst Environ Eng. 2015;50(14):1428-39. doi: 10.1080/10934529.2015.1074482. Epub 2015 Sep 1.

Abstract

This study aimed to compare and assess phthalate contamination in various indoor environments. In this study, 44 floor dust samples from different indoor environments in Delaware, USA were collected and analyzed for 14 phthalates using gas chromatography-mass spectrometry. Phthalates were detected in all dust samples with the total concentration ranging from 84 to 7117 mg kg(-1). DEHP (di-2-ethylhexyl phthalate), BzBP (benzylbutyl phthalate), DBP (dibutyl phthalate), and DiBP (di-isobutyl phthalate) were both the most frequently and abundantly detected phthalates. The average concentration of total phthalates in dust from offices, student dorms, gyms, stores, and daycare centers was found to be significantly or insignificantly (P = 0.05) higher than that in dust from houses and apartments. Plastic flooring materials and the application of floor care chemical products were positively associated with total phthalate concentration in floor dust. Toxicological risk assessment indicated that an investigated daycare center in this study was the only indoor environment that may cause the intake amount of DEHP of infants, toddlers, and children via dust ingestion to exceed the reference dose established by the U.S. Environmental Protection Agency (USEPA). Regular monitoring on phthalate contamination in sensitive indoor environments is recommended.

摘要

本研究旨在比较和评估不同室内环境中的邻苯二甲酸酯污染情况。在本研究中,采集了美国特拉华州不同室内环境的44份地板灰尘样本,并使用气相色谱 - 质谱法分析了14种邻苯二甲酸酯。所有灰尘样本中均检测到邻苯二甲酸酯,总浓度范围为84至7117 mg kg(-1)。邻苯二甲酸二(2-乙基己基)酯(DEHP)、邻苯二甲酸苄基丁酯(BzBP)、邻苯二甲酸二丁酯(DBP)和邻苯二甲酸二异丁酯(DiBP)是检测频率最高且含量最丰富的邻苯二甲酸酯。研究发现,办公室、学生宿舍、健身房、商店和日托中心灰尘中总邻苯二甲酸酯的平均浓度显著或不显著(P = 0.05)高于房屋和公寓灰尘中的浓度。塑料地板材料和地板护理化学产品的使用与地板灰尘中总邻苯二甲酸酯浓度呈正相关。毒理学风险评估表明,本研究中一个被调查的日托中心是唯一可能导致婴儿、幼儿和儿童通过灰尘摄入的DEHP摄入量超过美国环境保护局(USEPA)设定的参考剂量的室内环境。建议对敏感室内环境中的邻苯二甲酸酯污染进行定期监测。

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