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福岛第一核电站事故后放射性铯污染液体废物、土壤和灰烬的修复:一篇综述

Remediation of radiocesium-contaminated liquid waste, soil, and ash: a mini review since the Fukushima Daiichi Nuclear Power Plant accident.

作者信息

Ding Dahu, Zhang Zhenya, Lei Zhongfang, Yang Yingnan, Cai Tianming

机构信息

College of Resources and Environmental Sciences, Nanjing Agricultural University, No. 1 Weigang, Xuanwu District, Nanjing, 210095, China.

Graduate School of Life and Environmental Sciences, University of Tsukuba, Tsukuba, Ibaraki, 305-8572, Japan.

出版信息

Environ Sci Pollut Res Int. 2016 Feb;23(3):2249-63. doi: 10.1007/s11356-015-5825-4. Epub 2015 Nov 25.

DOI:10.1007/s11356-015-5825-4
PMID:26604196
Abstract

The radiation contamination after the Fukushima Daiichi Nuclear Power Plant accident attracts considerable concern all over the world. Many countries, areas, and oceans are greatly affected by the emergency situation other than Japan. An effective remediation strategy is in a highly urgent demand. Though plenty of works have been carried out, progressive achievements have not yet been well summarized. Here, we review the recent advances on the remediation of radiocesium-contaminated liquid waste, soil, and ash. The overview of the radiation contamination is firstly given. Afterwards, the current remediation strategies are critically reviewed in terms of the environmental medium. Special attentions are paid on the adsorption/ion exchange and electrically switched ion exchange methods. Finally, the present review outlines the possible works to do for the large-scale application of the novel remediation strategies.

摘要

福岛第一核电站事故后的辐射污染引起了全世界的广泛关注。除日本外,许多国家、地区和海洋都受到了这一紧急情况的严重影响。迫切需要一种有效的修复策略。尽管已经开展了大量工作,但尚未对取得的进展成果进行很好的总结。在此,我们综述了放射性铯污染液体废物、土壤和灰烬修复方面的最新进展。首先介绍了辐射污染的概况。然后,根据环境介质对当前的修复策略进行了批判性综述。特别关注了吸附/离子交换和电开关离子交换方法。最后,本综述概述了新型修复策略大规模应用可能需要开展的工作。

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本文引用的文献

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Design of Chitosan-Grafted Carbon Nanotubes: Evaluation of How the -OH Functional Group Affects Cs+ Adsorption.壳聚糖接枝碳纳米管的设计:-OH官能团对Cs+吸附影响的评估
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Predicting radiocaesium sorption characteristics with soil chemical properties for Japanese soils.
通过可压缩普鲁士蓝/聚氨酯海绵选择性去除铯离子的批次和固定床柱研究
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Enhanced irreversible fixation of cesium by wetting and drying cycles in soil.通过在土壤中进行润湿和干燥循环增强铯的不可逆转固定。
Environ Geochem Health. 2019 Feb;41(1):149-157. doi: 10.1007/s10653-018-0174-0. Epub 2018 Aug 24.
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Study of plasma off-gas treatment from spent ion exchange resin pyrolysis.研究废离子交换树脂热解产生的等离子体废气处理。
Environ Sci Pollut Res Int. 2018 Aug;25(22):21403-21410. doi: 10.1007/s11356-017-8766-2. Epub 2017 Mar 23.
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135Cs activity and 135Cs/137Cs atom ratio in environmental samples before and after the Fukushima Daiichi Nuclear Power Plant accident.福岛第一核电站事故前后环境样本中的¹³⁵Cs活度及¹³⁵Cs/¹³⁷Cs原子比。
Sci Rep. 2016 Apr 7;6:24119. doi: 10.1038/srep24119.
预测日本土壤中放射性铯的吸附特征与土壤化学性质的关系。
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