Department of Mechanical Engineering, University of Michigan, Ann Arbor, Michigan 48109, USA.
Departamento de Física Teórica de la Materia Condensada and Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, Madrid 28049, Spain.
Nature. 2015 Dec 17;528(7582):387-91. doi: 10.1038/nature16070. Epub 2015 Dec 7.
Radiative transfer of energy at the nanometre length scale is of great importance to a variety of technologies including heat-assisted magnetic recording, near-field thermophotovoltaics and lithography. Although experimental advances have enabled elucidation of near-field radiative heat transfer in gaps as small as 20-30 nanometres (refs 4-6), quantitative analysis in the extreme near field (less than 10 nanometres) has been greatly limited by experimental challenges. Moreover, the results of pioneering measurements differed from theoretical predictions by orders of magnitude. Here we use custom-fabricated scanning probes with embedded thermocouples, in conjunction with new microdevices capable of periodic temperature modulation, to measure radiative heat transfer down to gaps as small as two nanometres. For our experiments we deposited suitably chosen metal or dielectric layers on the scanning probes and microdevices, enabling direct study of extreme near-field radiation between silica-silica, silicon nitride-silicon nitride and gold-gold surfaces to reveal marked, gap-size-dependent enhancements of radiative heat transfer. Furthermore, our state-of-the-art calculations of radiative heat transfer, performed within the theoretical framework of fluctuational electrodynamics, are in excellent agreement with our experimental results, providing unambiguous evidence that confirms the validity of this theory for modelling radiative heat transfer in gaps as small as a few nanometres. This work lays the foundations required for the rational design of novel technologies that leverage nanoscale radiative heat transfer.
在纳米尺度上的能量辐射转移对于各种技术都非常重要,包括热辅助磁记录、近场热电和光刻技术。尽管实验上的进展已经能够阐明小至 20-30 纳米的近场辐射热传递[4-6],但在极端近场(小于 10 纳米)中的定量分析受到了实验挑战的极大限制。此外,开创性测量的结果与理论预测相差几个数量级。在这里,我们使用定制的嵌入热电偶的扫描探针,以及新的能够进行周期性温度调制的微器件,将辐射热传递测量到小至两个纳米的间隙。对于我们的实验,我们在扫描探针和微器件上沉积了适当选择的金属或介电层,从而能够直接研究二氧化硅-二氧化硅、氮化硅-氮化硅和金-金表面之间的极端近场辐射,揭示出辐射热传递的显著、间隙尺寸依赖性增强。此外,我们在波动电动力学理论框架内进行的辐射热传递的最先进计算与我们的实验结果非常吻合,这提供了明确的证据,证实了该理论对于建模小至几个纳米的间隙中的辐射热传递的有效性。这项工作为利用纳米尺度辐射热传递的新型技术的合理设计奠定了基础。