Amaladass E P, Devidas T R, Sharma Shilpam, Sundar C S, Mani Awadhesh, Bharathi A
Materials Science Group, IGCAR, Kalpakkam, TN 603102, India.
J Phys Condens Matter. 2016 Feb 24;28(7):075003. doi: 10.1088/0953-8984/28/7/075003. Epub 2016 Jan 26.
Magneto-resistance and Hall resistance measurements have been carried out in fast-cooled single crystals of Bi2Se3-xTex (x = 0 to 2) in 4-300 K temperature range, under magnetic fields up to 15 T. The variation of resistivity with temperature that points to a metallic behaviour in Bi2Se3, shows an up-turn at low temperatures in the Te doped samples. Magneto-resistance measurements in Bi2Se3 show clear signatures of Shubnikov-de Hass (SdH) oscillations that gets suppressed in the Te doped samples. In the Bi2SeTe2 sample, the magneto-resistance shows a cusp like positive magneto-resistance at low magnetic fields and low temperatures, a feature associated with weak anti-localisation (WAL), that crosses over to negative magneto-resistance at higher fields. The qualitatively different magneto-transport behaviour seen in Bi2SeTe2 as compared to Bi2Se3 is rationalised in terms of the disorder, through an estimate of the carrier density, carrier mobility and an analysis in terms of the Ioffe-Regel criterion with support from Hall Effect measurements. We demonstrate that by introducing Te, in the strongly disordered samples a smooth crossover of SdH and WAL can be seen in the Bi2Se3-xTex series, both of which provide signatures for the presence of topological surface states.
在4至300K的温度范围内,对Bi2Se3 - xTex(x = 0至2)的快速冷却单晶进行了磁阻和霍尔电阻测量,磁场强度高达15T。Bi2Se3中电阻率随温度的变化表明其具有金属行为,但在掺Te样品中,低温时出现了上扬。Bi2Se3中的磁阻测量显示出明显的舒布尼科夫 - 德哈斯(SdH)振荡特征,而在掺Te样品中这种振荡被抑制。在Bi2SeTe2样品中,磁阻在低磁场和低温下呈现出类似尖点的正磁阻,这一特征与弱反局域化(WAL)相关,在较高磁场时转变为负磁阻。通过估计载流子密度、载流子迁移率,并借助霍尔效应测量结果依据伊夫 - 雷格尔准则进行分析,将Bi2SeTe2与Bi2Se3相比在磁输运行为上的定性差异归因于无序性。我们证明,通过引入Te,在强无序样品中,Bi2Se3 - xTex系列中可以看到SdH和WAL的平滑转变,这两者都为拓扑表面态的存在提供了特征。