Advanced Technology Institute, University of Surrey, Guildford GU2 7XH, UK.
BAE Systems, Advanced Technology Centre, Sowerby Building (20R), FPC 267, P. O. Box 5, Filton, Bristol BS34 7QW, UK.
Sci Adv. 2016 Feb 26;2(2):e1501238. doi: 10.1126/sciadv.1501238. eCollection 2016 Feb.
The ability to engineer a thin two-dimensional surface for light trapping across an ultra-broad spectral range is central for an increasing number of applications including energy, optoelectronics, and spectroscopy. Although broadband light trapping has been obtained in tall structures of carbon nanotubes with millimeter-tall dimensions, obtaining such broadband light-trapping behavior from nanometer-scale absorbers remains elusive. We report a method for trapping the optical field coincident with few-layer decoupled graphene using field localization within a disordered distribution of subwavelength-sized nanotexturing metal particles. We show that the combination of the broadband light-coupling effect from the disordered nanotexture combined with the natural thinness and remarkably high and wavelength-independent absorption of graphene results in an ultrathin (15 nm thin) yet ultra-broadband blackbody absorber, featuring 99% absorption spanning from the mid-infrared to the ultraviolet. We demonstrate the utility of our approach to produce the blackbody absorber on delicate opto-microelectromechanical infrared emitters, using a low-temperature, noncontact fabrication method, which is also large-area compatible. This development may pave a way to new fabrication methodologies for optical devices requiring light management at the nanoscale.
在超宽光谱范围内实现光捕获的二维薄表面工程能力,对于越来越多的应用至关重要,包括能源、光电和光谱学。尽管已经在具有毫米级尺寸的碳纳米管高塔结构中获得了宽带光捕获,但从纳米级吸收体中获得这种宽带光捕获行为仍然难以实现。我们报告了一种使用亚波长尺寸的纳米纹理化金属颗粒的无序分布内的场局域化来捕获与少层解耦石墨烯重合的光场的方法。我们表明,无序纳米纹理的宽带光耦合效应与石墨烯的自然薄度和极高且波长独立的吸收相结合,导致超薄(15nm 厚)且超宽带黑体吸收体,具有从中红外到紫外的 99%吸收。我们展示了我们的方法在精密光电微机电红外发射器上产生黑体吸收体的实用性,使用低温、非接触制造方法,该方法还具有大面积兼容性。这一发展可能为需要在纳米尺度进行光管理的光学器件开辟新的制造方法。